COMPARISON OF THE DEPTH DISTRIBUTION PROCESSES FOR 137Cs AND lePbu IN CULTIVATED SOILS

探讨了^137Cs与^210Pbex在农耕地土壤深度分布过程的差异。基于^137Cs与^210Pbex的不同沉降过程,考虑到核素由犁耕层向犁底层的扩散,对农耕地土壤^137Cs与^210Pbex的深度分布过程进行了理论推导,并以杨凌符家庄麦田剖面的实测数据予以验证,同时讨论了实测符家庄麦田剖面^137Cs与^210Pbex深度分布的规律特征及其原因,以此阐明了^137Cs与^210Pbex在农耕地土壤深度分布过程的差异。^137Cs源于大气核试爆,没有持续沉降补充,犁耕层和犁底层土壤^137Cs深度分布一直处于随时间变化的非稳定态;而210Pbex是天然核素,存在大气沉降的持续补充,犁耕层和犁底层土壤^210Pbex深度分布最终呈稳定态。农耕地土壤^137Cs与^210Pbex深度分布的实测值曲线与理论值曲线的差异,尤其^210Pbex可能与耕作深度的变化历史或土地利用（覆被）变化有关。     

用 137Cs示踪法研究密云水库周边土壤侵蚀与氮磷流失

运用 ¹³⁷Cs核素示踪技术，研究密云水库周边地区及白河上游地区土壤侵蚀与氮、磷流失状况及其相互之间的量变关系。研究结果表明：从土壤表层(0～20 cm) ¹³⁷Cs分布规律基本符合地形地貌的变化规律，山坡上部的 ¹³⁷Cs含量低于山坡中部与坡下部，但是如果山顶具有缓坡或山角下具有陡坡，则 ¹³⁷Cs含量变化规律相反。根据土壤 ¹³⁷Cs监测数据结果判定该地区基本属于轻度侵蚀和中度侵蚀，部分地区侵蚀情况达到剧烈程度。不同景观与土地利用方式对土壤氮、磷分布有巨大影响：有机质、全氮、水解氮含量均是以灌丛土壤最高，林地次之，与流域内 ¹³⁷Cs分布规律相符合；而农田中全磷、速效磷含量最高。不同区域土壤养分含量不同：水库上游地区土壤氮素、磷素含量均低于水库周边地区。证明不合理的人为活动严重的增强了土壤侵蚀程度与养分流失量。回归模拟了土壤中 ¹³⁷Cs、( ²¹⁰Pb)与全氮、全磷、水解氮、速效磷含量之间的数学模型。这些模型在区域较小、景观单一的范围内可以定量分析、预报预测各采样区的全磷和有效态氮、磷含量的变化趋势。简化了监测与分析测试程序。扩大了核素示踪技术的应用范围。     

137Cs法测算梁峁坡农耕地土壤侵蚀量的初探

本文介绍了¹³⁷Cs法测算农耕地土壤侵蚀量的基本原理和方法。梁峁坡农耕地和梯田5个土壤剖面的¹³⁷Cs含量的测定结果表明,土壤剖面的¹³⁷Cs总量很好地表征了农耕地的侵蚀程度。根据卡钱诺斯基和奎因（Kachanoski and Quine）1987年分别提出的曲线和本文提出的公式求得的侵蚀模数值和实测资料分析值基本吻合。     

确定137Cs背景值所需的采样点数与采样面积

137Cs背景值的确定是利用核示踪技术研究土壤侵蚀的前提和根本,直接关系到侵蚀速率计算的准确与否。而大部分研究对137Cs背景值的确定均采取随机采样,没有统一的采样点数与确定的采样面积。本研究利用网格加密采样法,对未扰动地和长期耕种且未平整的农耕地各两块样地的137Cs背景值空间变异进行了分析,结果表明：在未扰动地与农耕地采样地块,137Cs采样点数与背景值空间变异系数都存在指数回归关系;在未扰动地块137Cs背景值存在较大空间变异性,且随着网格面积的扩大137Cs空间变异系数表现为增加趋势,在0.25m2范围内选取最少11个样点才能满足试验精度;在农耕地采样地块,因长期的耕种作用使得137Cs在耕层中混合相对均匀,137Cs背景值空间变异性显著变小,最少选取7个样点就能满足试验精度,且不受采样面积的影响。     

土壤呼吸及其13C同位素测定方法的对比研究

为比较不同方法在土壤呼吸及其_¹³C同位素测定中的差异，我们应用几种常见的方法测定了不同有机质含量的水稻土壤在一定时间内的CO₂排放量及_¹³C-CO₂丰度，以期准确评估土壤呼吸及碳排放，并为相关研究提供参考。本实验采用了气相色谱仪法(GC-TCD)、稳定同位素比值质谱仪气体进样法(Gasbench-IRMS)、甲酚红显色法(MicroResp)、碱液吸收法四种方法测定土壤呼吸速率；Gasbench-IRMS法和碱液吸收法两种方式检测土壤呼吸的_¹³CO₂含量。结果表明,(1)两种仪器法(GC、IRMS)测定土壤呼吸速率的数值结果相近(基础呼吸)或趋势一致(诱导呼吸),且重复性好（标准差分别为0.011、0.010 mg C /kg/h）,准确度高；MicroResp法的测定结果与仪器测量值较为相近,但分辨率较低；碱液吸收法的测定结果较真实值偏高(当土壤有机质含量低时)或偏低(当土壤有机质含量高时)。(2)在测定CO₂中的_¹³C含量上,Gasbench-IRMS直接测定的结果误差小(δ_¹³C值的标准偏差为0.137‰),接近实际值,可以准确地反应出土壤微生物呼吸时对底物的利用状况。综上,仪器法较化学分析法(MicroResp、碱液吸收)更能准确测定土壤呼吸及其_¹³C同位素。     

137Cs、HCHs测定岩溶洼地沉积物年代及流域产沙强度

以青木关岩溶槽谷区内代表性耕地型与林地型洼地小流域为研究对象,从洼地沉积物入手,探明各洼地沉积物剖面~(137)Cs比活度、六六六(HCHs)、有机质、黏粒含量及容重的深度分布特征;运用~(137)Cs示踪法,辅以HCHs进行沉积物断代,追溯流域近60年来的土壤侵蚀量演变特征及探讨其驱动因素。结果表明:(1)炮台院子耕地型洼地沉积物剖面~(137)Cs、HCHs仅有个别层位检出,无法利用~(137)Cs、HCHs深度分布进行沉积物断代,反映了发育的落水洞对其沉积物剖面影响大。(2)龙洞槽耕地型和劳动村林地型洼地小流域1963—1983,1984—2019年产沙模数分别为231.78,82.04 t/(km~2·a)和68.79,39.46 t/(km~2·a),表明流域生态环境得到明显改善。与1963—1983年时段相比,该地区1984—2019年时段年平均降水量无明显变化,2个小流域产沙模数均显著减小,表明近60年流域产沙强度主要受土地利用方式、水土保持措施等人类活动控制。(3)龙洞槽洼地剖面~(137)Cs、HCHs峰值,表层泥沙~(137)Cs、HCHs数值和不同时期流域产沙模数均明显大于劳动村洼地,主要是由2个洼地分别控制的耕地型与林地型小流域在人类活动影响下产沙强度的差异所致。另外,~(137)Cs和HCHs相结合的示踪方法可较好地用于评估西南岩溶流域产沙量的时间变化。     

强度耕作对137Cs、210Pbex和有机质剖面分布的影响

很少有关于直接测定强度耕作侵蚀引起土壤退化过程的报道.我们的目的是确定应用137Cs和210Pbex直接定量评价耕作侵蚀对土壤有机质(SOM)坡面运移影响的可能性.我们在黄土高原陡坡耕地上进行了50次犁耕活动,并将与其相临的另一块陡坡耕地作为对照.在对照坡地不同坡位,137Cs浓度均匀分布于上部0～30 cm土层,而210Pbex浓度在坡上部和坡中部随土层深度增加呈现线性递减,在坡下部呈指数函数递减.0～30 cm土层中土壤有机质含量显著大于30 cm深度以下土层,并在坡中部和坡下部呈现与210Pbex类似的土壤剖面分布特征.与对照坡地比较,50次犁耕活动导致坡上部、坡中部0～45 cm土层的SOM含量分别降低了38%和47%,坡下部0～100 cm土层中的SOM含量却提高了18%.坡上部土壤剖面中137Cs浓度的加权平均值从1.48 Bq/kg降低到0.29 Bq/kg, 坡中部从2.53 Bq/kg减少到0.33 Bq/kg,坡下部从1.48 Bq/kg提高到2.81 Bq/kg.210Pbex浓度的剖面加权平均值在坡上部从27.71 Bq/kg下降到6.15 Bq/kg,在坡中部和坡下部分别从35.46 Bq/kg和25.53 Bq/kg降低到1.57 Bq/kg和19.40 Bq/kg.137Cs和210Pbex的剖面分布与SOM在p<0.001水平呈显著相关,相关系数R2值在对照坡地为0.81～0.86,在犁耕实验坡地为0.86～0.91.实验结果表明,环境放射性核素137Cs和 210Pbex在黄土高原陡坡地遵照同一物理运移机理,可直接应用于定量评价耕作侵蚀与土壤质量的关系.     

紫色丘陵区小流域土壤侵蚀产沙空间分布的 137Cs法初步研究

该文通过紫色丘陵区响水滩小流域不同土地利用类型、不同坡度和坡长、不同地貌部位土壤剖面中 ¹³⁷Cs含量的测定与分析，对其侵蚀空间分布进行了估算。研究结果表明：该流域 ¹³⁷Cs含量的背景值为1870 Bq/m²；流域内坡耕地、林地的年平均侵蚀强度分别为4468、1759 t/(km²·a)；土壤侵蚀量与坡长、坡度均指数相关；丘顶、丘坡和鞍部的年平均侵蚀强度分别为2125、4676、3625 t/(km²·a)。结果表明土地利用类型、坡长和坡度、地貌部位对土壤侵蚀量影响很大，坡耕地是该流域泥沙的主要来源。     

基于137Cs的新疆准东地区不同土地利用类型 土壤风蚀特征研究

风力侵蚀是准东干旱与半干旱地区土地沙漠化的关键因素,通过野外考察和土壤~(137)Cs取样分析,对准东地区不同土地利用类型下土壤~(137)Cs分布特征及风力侵蚀进行了初步研究。研究表明,不同土地利用类型土壤~(137)Cs剖面分布特征不同,~(137)Cs基本分布在0~20 cm,甚至更浅,~(137)Cs活度值介于0~65.50 Bq/kg;各样点~(137)Cs总量介于0~1 698.29Bq/m~2,其中背景值为1 698.29 Bq/m~2,不同地类~(137)Cs总量排序为:低平地草甸(背景值样点)灌丛沙堆荒漠草地砾石戈壁盐碱地耕地固定沙地半固定沙地风蚀裸地;估算出耕地和非耕地各样点的风蚀速率,耕地平均风蚀速率为744.50 t/(km~2·a),非耕地风蚀速率介于945.06~4 404.01 t/(km~2·a)之间,平均值为2 589.96 t/(km~2·a)。     

黄土丘陵区典型沟道侵蚀诱发的CO2通量估算

以黄土丘陵区典型侵蚀沟道为对象,基于沟道剖面有机碳和¹³⁷Cs数据,采用碳库重分布模型估算了典型沟道侵蚀诱发的CO₂通量,并通过检验模型预测效率、解析影响因子,提出了模型校正的思路。结果表明:(1)在长期侵蚀作用下,沟道侵蚀区和沉积区均表现为剧烈的侵蚀效应,侵蚀区侵蚀速率介于30.99~46.44 mm/a,沉积区侵蚀速率介于34.20~37.88 mm/a,沉积区土壤流失速率略小于侵蚀区;(2)碳库重分布模型估算显示,侵蚀区与沉积区均表现为较强烈的碳源效应,侵蚀区CO₂通量介于18.41~28.44 g/(m²·a),沉积区CO₂通量介于22.19~29.25 g/(m²·a);(3)侵蚀部位、土壤容重、有机碳含量、侵蚀量、沟道平均坡度、植被地上部与地下部生物量共同解释了碳库重分布模型预测效率的变异特征(R²=0.68),其中侵蚀部位、侵蚀量、有机碳含量、土壤容重、植被地下部对预测效率有强驱动效应;(4)引入被忽略的植被新输入有机碳库参数,有望校正碳库重分布模型,提升模型预测效率。该研究结果明确了碳库重分布模型在沟道侵蚀区相比沉积区有更高的CO₂通量预测效率,为进一步提高模型的预测精度,可以考虑引入植被输入有机碳库作为校正参数。     

宁镇地区137Cs与210Pbex 坡面分布特征的地统计学分析

为更加深入地揭示核素示踪土壤侵蚀的内在机理,在Arcgis Geostatistics模块的支持下,运用地统计学方法研究了宁镇地区137Cs与210Pbex的空间异质性及其坡面分布特征。研究结果表明:(1)核素所特有的理化性质决定了137Cs与210Pbex的空间异质性及其坡面分布格局的与众不同。137Cs与210Pbex较大的块金值说明了土壤侵蚀及耕作活动等随机性因素对其空间分布的决定性影响,这正是它们能够示踪土壤侵蚀的原因所在。(2)137Cs属中等程度的空间自相关,其坡面分布格局能够较好地反映出地形这一结构性因素在其中所施加的影响,示踪土壤侵蚀的结果也应更为全面、合理,并具有宏观性。210Pbex的空间相关性很弱,说明其对随机性因素的影响有着更为敏感的响应,在揭示坡面侵蚀的细部特征方面应能做得更好。(3)137Cs与210Pbex坡面分布格局存在较大的差异,这一方面说明两者在初始沉降布局、部分理化性质,以及对各种变异影响因素的响应等诸多方面还存在着不小的差异;另一方面也在提示,两者示踪土壤侵蚀进程的结果很难通过数学模型的调整而达成一致。     

川中丘陵区人工刨地耕作方式下紫色土坡耕地侵蚀速率的137Cs和210Pbex双核素示踪法研究

Purple soils are widely distributed in the Sichuan Hilly Basin and are highly susceptible to erosion, especially on the cultivated slopes. Quantitative assessment of the erosion rates is, however, difficult due to small size of the plots of the manually-tilled land, the complex land use, and steep hillslopes. 137Cs and 210Pbex (excess 210Pb) tracing techniques were used to investigate the spatial pattern of soil erosion rates associated with slope-land under hoe tillage in Neijiang of the Sichuan Hilly Basin. The 137Cs and 210Pbex inventories at the top of the cultivated slope were extremely low, and the highest inventories were found at the bottom of the cultivated slope. By combining the erosion rates estimates provided by both 137Cs and 210Pbex measurements, the weighted mean net soil loss from the study slope was estimated to be 3100 t km-2 year-1, which was significantly less than 6930 t km-2 year-1 reported for runoff plots on a 10°cultivated slope at the Suining Station of soil Erosion. The spatial pattern of soil erosion rates on the steep agricultural land showed that hoe tillage played an important role in soil redistribution along the slope. Also, traditional farming practices had a significant role in reducing soil loss, leading to a lower net erosion rate for the field.     

137Cs和210Pbex双核素示踪"三北"防护林区退耕前后坡地土壤侵蚀变化

为查明"三北"防护林建设前后农耕地和退耕地土壤保持效益变化，利用137Cs和210Pbex双核素示踪技术，选择了防护林建设较为成功的张家口坝上地区（风力侵蚀区）作为典型区，研究了农耕地以及退耕地土壤137Cs和210Pbex的剖面变化规律及其示踪的土壤侵蚀变化。结果表明：1）由于耕作的混匀作用，农耕地土壤剖面中137Cs和210Pbex均呈均匀态分布；退耕地土壤剖面中137Cs和210Pbex则表现为表层（0～5cm）浓度最高、下层（5～25cm）浓度均相对较低且分布相对均匀的形态，这表明退耕后坡地土壤137Cs和210Pbex剖面形态均会发生一定变化，退耕驱动土壤137Cs和210Pbex剖面变化导致运用土壤核素估算侵蚀模型在该区域难以适用；2）基于土壤137Cs和210Pbex剖面变化规律，利用210Pbex质量平衡方程，提出了退耕地土壤210Pbex土壤侵蚀估算模型；3）利用137Cs比例模型估算退耕地土壤侵蚀速率为27.94±11.92 (t/hm2·a)，农耕地侵蚀速率为29.11±14.42 (t/hm2·a)，而利用修正后的210Pbex转换模型估算得到"三北"防护林区退耕地造林前平均侵蚀速率为82.16±14.36 (t/hm2·a)，造林后平均侵蚀速率为-41.28±33.91 (t/hm2·a)；农耕地造林前平均侵蚀速率为68.55±22.11 (t/hm2·a)，造林后平均侵蚀速率-8.52±47.32 (t/hm2·a)。这表明137Cs示踪技术主要表征了1963年以来该区坡地土壤侵蚀和沉积的平均结果，而210Pbex示踪技术则可以较好地示踪防护林建成前后的土壤侵蚀变化。此外，研究结果也表明，相比于"三北"防护林建成之前，建成之后该区农耕地和退耕地的土壤侵蚀速率均呈显著下降趋势，且均由前期的风沙侵蚀转变成了风沙沉积。     

用137Cs和210Pbex进行中国东北地区土壤侵蚀的评估

Evaluation of soil erosion in agricultural fields is valuable to develop conservation practices for reducing agricultural nonpoint source pollution.Soil erosion rates were quantified using the fallout radionuclide tracer technique in Mojiagou Basin located on the outskirts of Changchun in Northeast China.The calculated soil erosion rates in the study area were 1.99 and 1.85 mm year-1 using 137Cs and excess 210Pb(210Pbex)measurements,respectively.Both fallout radionuclides showed a similar tendency at downslope sites.All measured sites have experienced net erosion during the past 50 to 100 years.137Cs and 210Pbex measurements were useful to quantify soil erosion rates on field and small basin scales.At this rate of erosion,the current fertile topsoil layer would be entirely removed within 70 years.     

中国西南薄层砾石土喀斯特坡地土壤的137Cs分布特点

The fallout radionuclide cesium-137(137 Cs) has been widely employed as a tracer for assessment of soil loss from thick uniform soils;however,few studies have been conducted on thin stony soils on slopes underlain by carbonate rocks which are widely distributed in karst areas.Information derived from 137 Cs measurement of soil samples collected along a carbonate rock slope with thin stony soil where neither soil erosion nor deposition occurred was used to investigate the characteristics of 137 Cs redistribution in a karst area of Southwest China.The results indicated that the 137 Cs inventories of the surface soil on the slope studied were much lower than that of the local 137 Cs reference inventory and the 137 Cs activities were much higher than those on slopes with thick uniform soils.The spatial distribution of 137 Cs inventories was characterized by considerable variation.The high 137 Cs depletion in the stony soil of the slope studied was mainly because a considerable proportion of the fallout input of 137 Cs could be lost with runoff and the dissolution of carbonate particles in the soil promoted the loss of 137 Cs.These demonstrated that the rates of soil loss could not be estimated from the degree of depletion of the 137 Cs inventory relative to the local reference inventory for the thin stony soil of the rocky slope underlain by carbonate rocks in the study area in the way that has been widely used in areas with thick uniform soils.     

~(137)Cs在土壤中的污染行为与钾盐的防治效果

本研究结果表明 ,在污染水平相同的情况下 ,不同土壤对春小麦吸收137Cs有很大影响 ,植株中137Cs的比活度相差几十倍。在同一种土壤、不同污染水平下 ,春小麦对137Cs的吸收与土壤中137Cs的污染水平呈正相关。在137Cs污染的土壤上施用钾盐可以降低春小麦植株对137Cs的吸收。防治效果与钾盐施用量有关 ,本试验结果为土壤阳离子代换量 1 / 3 0的量施用效果最好 ,使植株中的137Cs比活度降低 84 74%～88 89% ,与不施钾盐的对照组的差异十分显著     

基于137Cs的土壤沉积速率的定量模型

在假设137Cs在耕层中得到充分混合而变得均一的基础上,根据质量平衡原理建立了一个根据农业耕作土壤剖面中137Cs的沉积量和土壤沉积量之间关系的定量模型.在建立模型的过程中,充分考虑了137Cs的衰变常数,年沉降分量,耕层厚度和采样年份等因素.模型的模拟结果表明,137Cs的沉积量与年平均土壤沉积量之间的关系是一种复杂的曲线关系.     

利用137Cs估算土壤侵蚀速率的定量模型

A quantitative model was developed to relate the amount of ^137Cs loss from the soil profile to the rate of soil erosion,According th mass balance model,the depth distribution pattern of ^137Cs in the soil profile ,the radioactive decay of ^137Cs,sampling year and the difference of ^137Cs fallout amount among years were taken into consideration.By introducing typical depth distribution functions of ^137Cs into the model ,detailed equations for the model were got for different soil,The model shows that the rate of soil erosion is mainly controlled by the depth distrbution pattern of ^137Cs ,the year of sampling,and the percentage reduction in total ^137Cs,The relationship between the rate of soil loss and ^137Cs depletion i neither linear nor logarithmic,The depth distribution pattern of ^137Cs is a major factor for estimating the rate of soil loss,Soil erosion rate is directly related with the fraction of ^137Cs content near the soil surface. The influences of the radioactive decay of ^137Cs,sampling year and ^137Cs input fraction are not large compared with others.     

A preliminary assessment of the potential for using Pbex measurement to estimate soil redistribution rates on cultivated slopes in the Sichuan Hilly Basin of China

In order to assess its potential for estimating soil redistribution rates, the naturally occurring fallout radionuclide ²¹⁰Pb_ex has been used in parallel with ¹³⁷Cs, derived from the atmospheric testing of nuclear weapon testing in the 1950s to 1970s, to estimate rates of soil redistribution on a sloping field with traditional erosion control measures located near Jiajia Village, Jianyang County, in the Sichuan Hilly Basin of China. The local ²¹⁰Pb_ex reference inventory of 12,860 Bq m^− 2 is higher than those reported for many other areas of the world and may reflect the influence of cloudy weather in preventing ²¹⁰Pb released to the atmosphere across the local region moving up into the upper troposphere, where is would be more widely dispersed. The mean ²¹⁰Pb_ex and ¹³⁷Cs inventories measured in cores collected from the upper part of the field with an average slope of 10° were 8028 Bq m^− 2 and 993 Bq m^− 2, respectively, and the equivalent values for the lower part of the field, where the slopes are steeper (20°) were 11,388 Bq m^− 2 and 1299 Bq m^− 2. The pattern of post-fallout ²¹⁰Pb_ex and ¹³⁷Cs redistribution on the sloping field reflects not only the effects of water erosion and redistribution by tillage, but also the local traditional practice of “Tiaoshamiantu”, whereby sediment trapped in the ditches is returned to the fields by the farmer. The estimates of annual rates of soil loss provided by the ²¹⁰Pb_ex measurement are closely comparable with those derived from the ¹³⁷Cs measurements and are consistent with existing knowledge for the study area. The results obtained from this study confirm the potential for using ²¹⁰Pb_ex measurement to estimate soil erosion rates over medium-term timescale of 50–100 years. By combining the estimates of erosion rates provided by the ²¹⁰Pb_ex and ¹³⁷Cs measurements, the weighted mean net soil loss was estimated to be 48.7 t ha^− 1 year^− 1 from the upper subfield and 16.9 t ha^− 1 year^− 1 from the lower subfield. These rates are considerably lower than the erosion rates obtained from runoff plot measurements in the local area. It is suggested that the traditional erosion control practices and the practice of “Tiaoshamiantu” have a significant effect in reducing soil loss and conserving valuable cultivated soil on sloping fields in the Sichuan Hilly Basin.     

贵州省西南部麦岗水库沉积物的137Cs和210Pb测年与沉积速率研究

对贵州省西南部麦岗水库沉积物柱芯MG4-2,采用210Pb和137Cs法进行了测年与现代沉积速率研究.结果表明,该柱芯中存在这3个明显的137Cs蓄积峰,对应1964,1975,1986年3个计年时标.运用210Pb的恒定补给速率(CRS)模式计算得到的年代,总体上与137Cs法的结果吻合较好,但存在一定的偏差,特别是与1964年的计年时标的偏差较大,这可能是因为沉积物柱芯受到了一些人为扰动所致.两种核素测定的平均沉积速率在数值上有一定的偏差,但都反映了麦岗水库沉积物近几十年以来经历了从慢到快再到慢的沉积过程,初步推测,沉积速率的这种变化与人类活动有一定的关系.两种计年方法结合,相互印证,使计年和沉积速率的研究更为准确.