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Historical sediment mercury deposition for select South Dakota,USA, lakes: implications for watershed transport and flooding |
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| Authors: | Squillace Maria K Sieverding Heidi L Betemariam Hailemelekot H Urban Noel R Penn Michael R DeSutter Thomas M Chipps Steven R Stone James J |
| Institution: | 1.Department of Civil and Environmental Engineering, South Dakota School of Mines and Technology, Rapid City, SD, 57701, USA ;2.Department of Geology and Geological Engineering, South Dakota School of Mines and Technology, Rapid City, SD, 57701, USA ;3.Department of Civil and Environmental Engineering, Michigan Technological University, Houghton, MI, 49931, USA ;4.Department of Civil Engineering, University of Wisconsin-Platteville, Platteville, WI, 53818, USA ;5.Department of Soil Science, North Dakota State University, Fargo, ND, 58108, USA ;6.U.S. Geological Survey, South Dakota Cooperative Fish and Wildlife Research Unit, Department of Wildlife and Fisheries Sciences, South Dakota State University, Brookings, SD, 57007, USA ; |
| Abstract: | Purpose Select South Dakota, USA water bodies, including both natural lakes and man-made impoundments, were sampled and analyzed to assess mercury (Hg) dynamics and historical patterns of total Hg deposition. Materials and methodsSediment cores were collected from seven South Dakota lakes. Mercury concentrations and flux profiles were determined using lead (210Pb) dating and sedimentation rates. Results and discussionMost upper lake sediments contained variable heavy metal concentrations, but became more consistent with depth and age. Five of the seven lakes exhibited Hg accumulation fluxes that peaked between 1920 and 1960, while the remaining two lakes exhibited recent (1995–2009) Hg flux spikes. Historical sediment accumulation rates and Hg flux profiles demonstrate similar peak and stabilized values. Mercury in the sampled South Dakota lakes appears to emanate from watershed transport due to erosion from agricultural land use common to the Northern Great Plains. ConclusionsFor sampled South Dakota lakes, watershed inputs are more significant sources of Hg than atmospheric deposition. |
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