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151.
Thanh Thuy Nguyen Tu Céline Egasse Gérard Bardoux Jean-François Ponge Sylvie Derenne 《Soil biology & biochemistry》2011,43(11):2222-2228
We monitored the carbon isotope composition of bulk leaves and specific long-chain alkanes during a four-year litterbag experiment using 13C-labelled leaves and unlabelled reference leaves of the European beech tree (Fagus sylvatica L.). Whereas the isotope composition of alkanes from 13C-enriched leaves exhibited a marked decrease in 13C-content, the isotope composition of unlabelled reference leaves remained nearly constant. We interpreted this difference as evidence for a microbial contribution to the long-chain alkane pool of the decomposing leaves and related it to the progressive invasion of leaves by soil organisms which was revealed upon microscopic examination. These results suggest that long-chain alkanes may not provide an unaltered record of organic carbon isotope composition in soils and sediments. 相似文献
152.
The present study focuses on the microbial recalcitrance of pyrogenic organic material (PyOM) on a molecular scale. We performed microcosm incubation experiments using 13C- and 15N-enriched grass-derived PyOM mixed with a sub soil material taken from a Haplic Cambisol. Solid-state 13C and 15N NMR studies were conducted to elucidate the humification processes at different stages of PyOM degradation. The chemical structure of the remaining PyOM after incubation was clearly different from the initial pyrogenic material. The proportion of O-containing functional groups was increased, whereas that of aryl C and of N-containing heterocyclic structures had decreased, probably due to mineralisation and conversion to other C and N groups. After 20 months of incubation the aryl C loss reached up to 40% of the initial amount and up to 29% of the remaining PyOM C was assigned to carboxyl/carbonyl C and O-aryl C. These reactions alter the chemical and physical properties of the char residue and make it more available for further microbial attack but also for adsorption processes. Our study presents direct evidence for the degradation of N-heterocyclic domains in charred plant remains adding new aspects to the understanding of the N cycling in fire-affected ecosystems. 相似文献
153.
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155.
Paul Dijkstra Ayaka Ishizu Stephen C. Hart Egbert Schwartz Bruce A. Hungate 《Soil biology & biochemistry》2006,38(11):3257-3266
Stable isotope analysis is a powerful tool in the study of soil organic matter formation. It is often observed that more decomposed soil organic matter is 13C, and especially 15N-enriched relative to fresh litter and recent organic matter. We investigated whether this shift in isotope composition relates to the isotope composition of the microbial biomass, an important source for soil organic matter. We developed a new approach to determine the natural abundance C and N isotope composition of the microbial biomass across a broad range of soil types, vegetation, and climates. We found consistently that the soil microbial biomass was 15N-enriched relative to the total (3.2 ‰) and extractable N pools (3.7 ‰), and 13C-enriched relative to the extractable C pool (2.5 ‰). The microbial biomass was also 13C-enriched relative to total C for soils that exhibited a C3-plant signature (1.6 ‰), but 13C-depleted for soils with a C4 signature (−1.1 ‰). The latter was probably associated with an increase of annual C3 forbs in C4 grasslands after an extreme drought. These findings are in agreement with the proposed contribution of microbial products to the stabilized soil organic matter and may help explain the shift in isotope composition during soil organic matter formation. 相似文献
156.
西伯利亚落叶松树轮稳定碳同位素对气候的响应 总被引:2,自引:0,他引:2
利用采自阿尔泰山南坡东段正格采点的西伯利亚落叶松树轮样本,建立树轮宽度年表,对比宽度年表,按照树轮稳定碳同位素研究步骤,提取树轮稳定碳同位素序列(δ13C)和去趋势序列(DS)。分析表明:阿尔泰山南坡东部近160 a西伯利亚落叶松树轮δ13C变化于-22.8‰~-25.4‰,平均值为-24.0‰,变差系数-0.017。相关分析表明:正格采点树轮宽度序列对各气候要素相关不显著;树轮去趋势序列(DS)对前期气候因子的响应也不敏感;在生长季内(5~9月),树轮去趋势序列(DS)与富蕴气象站平均气温、平均最高气温和平均相对湿度有较好的相关性,树木生长季内的平均气温、平均最高气温与树轮去趋势序列(DS)显著正相关,6~7月平均最高气温与去趋势序列(DS)相关达到0.611(P<0.000 001);与生长季内平均相对湿度呈负相关关系,其中6~7月相对湿度与去趋势序列(DS)相关最高(r=-0.493, P<0.001),与7月降水量呈负相关关系(r=-0.459, P<0.01)。生长季内的平均最高气温和相对湿度对阿尔泰山西伯利亚落叶松树轮δ13C的响应最为敏感,阿尔泰山西伯利亚落叶松树木碳同位素分馏的主要控制因子为6~7月的平均最高气温,降水对树轮稳定碳同位素影响不大,相对湿度对树轮稳定碳同位素没有直接影响。 相似文献
157.
为开展碳、氮、氢、氧(C、H、O、N)稳定同位素鉴别库尔勒香梨产地的可行性研究,明确新疆库尔勒香梨δ13C、δ15N、δ2H、δ18O值,本研究以甘肃香梨和陕西红香酥梨作为对照,采用稳定同位素比值质谱仪(IRMS)分析新疆库尔勒香梨与对照样品的δ13C、δ15N、δ2H、δ18O值,并采用正交校正的偏最小二乘判别分析(OPLS-DA) 鉴别新疆库尔勒香梨产地真实性。结果表明,新疆、甘肃两个产区香梨与陕西产区红香酥梨的δ13C、δ15N、δ2H、δ18O值存在显著差异(P<0.05)。新疆产区的66份库尔勒香梨判别准确率为95.45%;甘肃产区的20份香梨样品判别准确率为60%;陕西产区的23份红香酥梨样品判别准确率为95.65%。C、N、H、O 4种稳定同位素可有效鉴别新疆库尔勒香梨和陕西红香酥梨,但在新疆库尔勒香梨与甘肃香梨鉴别方面,误判率较高,如果能结合其他鉴别技术,则有可能出现较好的鉴别效果。本研究为库尔勒香梨产地真实性鉴别提供了科学依据。 相似文献
158.
中国西北中小型盆地天然地下水水化学特征——以公婆泉盆地为例 总被引:2,自引:1,他引:2
研究分析干旱气候条件下甘肃北山公婆泉盆地天然地下水水化学成分特征,结合水文地质条件与水化学特征Piper三线图表明:研究区存在4种类型地下水,白垩系深层水中钙镁离子含量相对高于其他类型水.地下水氚同位素结合水化学特征较好地区分了水源点的水文地质属性.氢氧同位素表明,该区地下水来源于大气降水,第四系浅层水受到强烈的蒸发作用,发生了一定程度的氧漂移,并影响"混合水"的同位素组成.最后分析了地下水主要离子的来源,以及地下水形成过程中所受到的溶滤、沉积和蒸发等水文地球化学作用. 相似文献
159.
Owing to the continuously increasing concentration of atmospheric CO2, it has become a priority to understand if soil organic matter (SOM) will behave as a sink or a source of CO2 under future environmental changes. Although many studies have addressed this question, a clear understanding is still missing, particularly with respect to long-term responses. In this study, we quantified soil C stores and dynamics in relationship to soil aggregation and pool composition in a Californian chaparral ecosystem exposed for 6 years to a gradient of atmospheric CO2 concentrations, ranging from pre-industrial levels 250 to 750 μl l−1 CO2. Fossil fuel-derived CO2 depleted in 13C was used for the fumigation, thus providing a tracer of C input from the vegetation to the soil.Long-term CO2 exposure invariably affected soil aggregation, with a significant decrease in the macroaggregate fraction at highest CO2 levels relative to the other two size fractions (i.e. microaggregates and silt and clay). This soil structural change most likely reduced the stability and protection of SOM, and C content generally decreased in most fractions over the CO2 treatments, and induced faster turnover of recently fixed C at high CO2 levels. The strongest response was found in the C content of the microaggregates, which decreased significantly (P<0.05) with rising levels of CO2. We conclude that increasing atmospheric CO2 concentrations will decrease soil C in chaparral ecosystems, and that the microaggregate fraction is the most responsive to increasing concentrations of atmospheric CO2. 相似文献
160.
Mehmet Senbayram Roland Bol Liz Dixon Andrew Fisher Carly Stevens John Quinton David Fangueiro 《植物养料与土壤学杂志》2015,178(2):288-296
Tracing organic matter (OM) in soil is challenging, because runoff and leaching processes are interrelated and have multiple sources. Therefore, multiple tracers with low background concentrations such as rare earth element oxides (REOs) are necessary to delineate the origin of sources of the organic materials in groundwater, rivers or in catchments. The main objective of this study was to examine the potential use of REOs as a tracer in various forms of OM (1) whole slurry, (2) solid, and (3) liquid phase of cattle slurry after mechanical separation. A laboratory experiment was carried out using five REOs (La, Gd, Sm, Pr, and Nd oxides) mixed directly into soil or mixed with various fractions of cattle slurry and then applied to the soil surface. In the additional grassland experiment, Gd oxide was spiked with soil and cattle slurry and then applied to the soil surface. The mineral N in the liquid phase (urine) of the slurry in the grassland experiment was labelled with 15N urea (16 atom%). In the laboratory experiment, results showed that the five REOs concentration of soil in 0–1 cm soil section after the rainfall simulation was still up to 20 times more than the background values. In 1–2 cm soil section, the concentration of only Gd (two fold higher) and La oxides (50% higher) were significantly higher than the soil background values. Therefore, we hypothesized that Gd and La oxides were associated also with relatively finer organic particles in slurry, thus 1–2 cm soil section were enriched with these oxides. The five REOs concentration below 2 cm soil depth were similar to the background values in all treatments. In line with the laboratory experiment, Gd concentrations in the deeper soil layers (2–4 and 4–8 cm) in the grassland experiment were not significantly affected by any treatment. Both in grassland and laboratory experiment, solid phase of the slurry (dung) was collected from the soil surface after rainfall simulation. Here, about 56% of REOs were measured on the solid phase of the slurry which indicates the strong binding potential of REOs on slurry OM. The present novel study, where REO tagged slurry was uniquely tested to study geochemical cycle of organic fertilizers, clearly highlighted the potential for their use as multiple‐tracers of (animal derived‐) OM in agricultural soils. 相似文献