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Mercury in the Swedish environment — Recent research on causes,consequences and corrective methods 总被引:3,自引:0,他引:3
Oliver Lindqvist Kjell Johansson Lage Bringmark Birgitta Timm Mats Aastrup Arne Andersson Gunnar Hovsenius Lars Håkanson Åke Iverfeldt Markus Meili 《Water, air, and soil pollution》1991,55(1-2):xi-261
During the last decade a new pattern of Hg pollution has been discerned, mostly in Scandinavia and North America. Fish from low productive lakes, even in remote areas, have been found to have a high Hg content. This pollution problem cannot be connected to single Hg discharges but is due to more widespread air pollution and long-range transport of pollutants. A large number of waters are affected and the problem is of a regional character. The national limits for Hg in fish are exceeded in a large number of lakes. In Sweden alone, it has been estimated that the total number of lakes exceeding the blacklisting limit of 1 mg Hg kg-1 in 1-kg pike is about 10 000. The content of Hg in fish has markedly increased in a large part of Sweden, exceeding the estimate background level by about a factor of 2 to 6. Only in the northernmost part of the country is the content in fish close to natural values. There is, however, a large variation of Hg content in fish within the same region, which is basically due to natural conditions such as the geological and hydrological properties of the drainage area. Higher concentrations in fish are mostly found in smaller lakes and in waters with a higher content of humic matter. Since only a small percentage of the total flow of Hg through a lake basin is transferred into the biological system, the bioavailability and the accumulation pattern of Hg in the food web is of importance for the Hg concentrations in top predators like pike. Especially, the transfer of Hg to low trophic levels seems to be a very important factor in determining the concentration in the food web. The fluxes of biomass through the fish community appear to be dominated by fluxes in the pelagic food web. The Hg in the lake water is therefore probably more important as a secondary source of Hg in pike than is the sediment via the benthic food chain. Different remedy actions to reduce Hg in fish have been tested. Improvements have been obtained by measures designed to reduce the transport of Hg to the lakes from the catchment area, eg. wetland liming and drainage area liming, to reduce the Hg flow via the pelagic nutrient chains, eg. intensive fishing, and to reduce the biologically available proportion of the total lake dose of Hg, eg. lake liming with different types of lime and additions of selenium. The length of time necessary before the remedy gives result is a central question, due to the long half-time of Hg in pike. In general it has been possible to reduce the Hg content in perch by 20 to 30% two years after treatments like lake liming, wetland liming, drainage area liming and intensive fishing. Selenium treatment is also effective, but before this method can be recommended, dosing problems and questions concerning the effects of selenium on other species must be evaluated. Regardless how essential these kind of remedial measures may be in a short-term perspective, the only satisfactory long-term alternative is to minimize the Hg contamination in air, soil and water. Internationally, the major sources of Hg emissions to the atmosphere are chlor-alkali factories, waste incineration plants, coal and peat combustion units and metal smelter industries. In the combustion processes without flue gas cleaning systems, probably about 20 to 60% of the Hg is emitted in divalent forms. In Sweden, large amounts of Hg were emitted to the atmosphere during the 50s and 60s, mainly from chlor-alkali plants and from metal production. In those years, the discharges from point sources were about 20 to 30 t yr 1. Since the end of the 60s, the emission of Hg has been reduced dramatically due to better emission control legislation, improved technology, and reduction of polluting industrial production. At present, the annual emissions of Hg to air are about 3.5 t from point sources in Sweden. In air, more than 95% of Hg is present as the elemental Hg form, HgO0. The remaining non-elemental (oxidized) form is partly associated to particles with a high wash-out ratio, and therefore more easily deposited to soils and surface waters by precipitation. The total Hg concentration in air is normally in the range 1 to 4 ng m-3. In oceanic regions in the southern hemisphere, the concentration is generally about 1 ng m?3, while the corresponding figure for the northern hemisphere is about 2 ng m-3. In remote continental regions, the concentrations are mainly about 2 to 4 ng m?3. In precipitation, Hg concentrations are generally found in the range 1 to 100 ng L?1. In the Nordic countries, yearly mean values in rural areas are about 20 to 40 ng L?1 in the southern and central parts, and about 10 ng L?1 in the northern part. Accordingly, wet deposition is about 20 (10 to 35) g km?2 yr?1 in southern Scandinavia and 5 (2 to 7) in the northern part. Calculations of Hg deposition based on forest moss mapping techniques give similar values. The general pattern of atmospheric deposition of Hg with decreasing values from the southwest part of the country towards the north, strongly suggests that the deposition over Sweden is dominated by sources in other European countries. This conclusion is supported by analyses of air parcel back trajectories and findings of significant covariations between Hg and other long range transported pollutants in the precipitation. Apart from the long range transport of anthropogenic Hg, the deposition over Sweden may also be affected by an oxidation of elemental Hg in the atmosphere. Atmospheric Hg deposited on podzolic soils, the most common type of forest soil in Sweden, is effectively bound in the humus-rich upper parts of the forest soil. In the Tiveden area in southern Sweden, about 75 to 80% of the yearly deposition is retained in the humus layer, chemically bound to S or Se atoms in the humic structure. The amount of Hg found in the B horizon of the soils is probably only slightly influenced by anthropogenic emissions. In the deeper layers of the soil, hardly any accumulation of Hg takes place. The dominating horizontal flow in the soils takes place in the uppermost soil layers (0 to 20 cm) during periods of high precipitation and high groun water level in the soils. The yearly transport of Hg within the soils has been calculated to be about 5 to 6 g km?2. The specific transport of total Hg from the soil system to running waters and lakes in Sweden is about 1 to 6 g km?2 yr1. The transport of Hg is closely related to the transport of humic matter in the water. The main factors influencing the Hg content and the transport of Hg in run-off waters from soils are therefore the Hg content in soils, the transport of humic matter from the soils and the humus content of the water. Other factors, for example acidification of soils and waters, are of secondary importance. Large peatlands and major lake basins in the catchment area reduce the out-transport of Hg from such areas. About 25 to 75% of the total load of Hg of lakes in southern and central Sweden originates from run-off from the catchment area. In lakes where the total load is high, the transport from run-off is the dominating pathway. The total Hg concentrations in soil solution are usually in the range 1 to 50, in ground water 0.5 to 15 and in run-off and lake water 2 to 12 ng L?1, respectively. The variation is largely due to differences in the humus content of the waters. In deep ground water with a low content of humic substances, the Hg concentration is usually below 1 ng L?1. The present amount and concentrations of Hg in the mor layer of forest soils are affected by the total anthropogenic emissions of Hg to the atmosphere, mainly during this century. Especially in the southern part of Sweden and in the central part along the Bothnian coast, the concentrations in the mor layer are markedly high. In southern areas the anthropogenic part of the total Hg content is about 70 to 90%. Here, the increased content in these soils is mainly caused by long-range transport and emissions from other European countries, while high level areas in the central parts are markedly affected by local historical emissions, mainly from the chlor-alkali industry. When comparing the input/output fluxes to watersheds it is evident that the present atmospheric deposition is much higher than the output via run-off waters, on average about 3 to 10 times higher, with the highest ration in the southern parts of Sweden. Obviously, Hg is accumulating in forest soils in Sweden at the present atmospheric deposition rate and, accordingly, the concentrations in forest soils are still increasing despite the fact that the emissions of Hg have drastically been reduced in Sweden during the last decades. The increased content of Hg in forest soils may have an effect on the organisms and the biological processes in the soils. Hg is by far the most toxic metal to microorganisms. In some regions in Sweden, the content of Hg in soils is already today at a level that has been proposed as a critical concentration. To obtain a general decrease in the Hg content in fish and in forest soils, the atmospheric deposition of Hg has to be reduced. The critical atmospheric load of Hg can be defined as the load where the input to the forest soils is less than the output and, consequently, where the Hg content in the top soil layers and the transport of Hg to the surface waters start to decrease. A reduction by about 80% of the present atmospheric wet deposition has to be obtained to reach the critical load for Scandinavia. 相似文献
13.
不同比例尺DEM提取地面坡度的精度研究——以在黄土丘陵沟壑区的试验为例 总被引:53,自引:8,他引:53
以陕北绥德县韭园沟流域为试验样区 ,采用高精度 1∶ 1万 DEM所提取的坡度为准值 ,应用多层面复合分析和比较分析的方法 ,研究该地区 1∶ 5万 DEM提取地面坡度的误差特征与纠正方法。试验结果显示 ,所获得的不同空间尺度下 DEM所提取坡度值的转换图谱 ,可对 1∶ 5万 DEM计算的地面坡度统计值进行有效修正。该成果对于 DEM数据在水土保持领域若干应用标准的制定 ,提供了重要的理论依据与技术路线 相似文献
14.
干旱胁迫下沙棘膜脂过氧化保护体系研究 总被引:56,自引:1,他引:56
研究了干旱胁迫下沙棘幼林苗木自由基清除系统活性与沙棘耐旱性的关系.结果表明:长期轻度及中度干旱胁迫下保护酶系统SOD、POD、CAT活性均高于正常水平,重度干旱下3种酶活性均能在胁迫初期随时间延长而上升;抗氧化物质AsA在轻度、中度干旱下高于对照,GSH含量在轻度干旱下含量与对照接近,中度及重度干旱下前、中期随时间延长趋于增加,而后期降低,表明干旱下自由基清除系统活性高,能有效减轻膜脂过氧化伤害,细胞膜透性和MDA含量增加不明显.由于沙棘保护酶体系(SOD、POD、CAT)、抗氧化物质(AsA、GSH)、细胞膜透性和MDA含量增加缓慢,重度干旱下也能在一定时间内保持稳定,这些物质是构成沙棘强耐旱性的内在基础. 相似文献
15.
鸡柔嫩艾美耳球虫单卵囊分离技术的构建及致病性研究 总被引:16,自引:3,他引:16
构建了一种新的鸡柔嫩艾美耳球虫单卵囊分离技术 ,并对杨陵柔嫩艾美耳球虫地理株进行了分离 ,对继代增殖的纯种卵囊进行了致病性试验。结果表明 ,该单卵囊分离技术简单易行 ,单卵囊感染成功率可达4 0 % ;该虫株对雏鸡有很强的致病性 ,经口接种 1× 10 5个孢子化卵囊 ,致死率高达 80 %。 相似文献
16.
17.
抗日战争时期,陕甘宁边区的奶业方兴未艾。以光华农场为代表的奶业科研及生产机构,大力开展奶畜育种、饲养、管理、防疫等方面的科研工作,试验制作奶酪、奶皮、奶油、酸奶等奶制品,成为了边区奶业的技术扩散源。抗日军民对牛、羊奶的大量需求,客观上促进了边区奶业技术的传播与辐射,但受经济条件、饮食习惯以及市场流通等多重因素的影响和制约,边区奶业技术扩散呈现出比较复杂的情形。 相似文献
18.
P. Nilsson Sven‐Åke Johansson Arnulf Merker 《Acta Agriculturae Scandinavica, Section B - Plant Soil Science》2013,63(3):159-164
The seed oil composition and content in a number of accessions from species of the genera Barbarea and Lepidium were analysed. The oil from most accessions of B. verna contained more than 50% erucic acid, while the oil from B. vulgaris contained ~ 30% erucic acid, and 22% each of oleic and linoleic acid. The oil from B. intermedia resembled that of B. verna. The oil content was ~ 30% in all three species. The oil composition of L. campestre and L. heterophyllum is ~ 35% linolenic acid and 23% erucic acid. Other Lepidium species had up to 47% linolenic acid in the oil. The oil content of L. campestre and L. heterophylhim was just below 20%, but other species had more than 30% oil in their seeds. The variation in oil composition found within and between species is considered sufficient for the breeding of valuable oil qualities in both genera. 相似文献
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江苏仪征低丘岗地营林开发模式优化选择研究 总被引:4,自引:3,他引:4
总结江苏省仪征低丘岗地开发的经济林、用材林等7种营林模式和5种纯板栗与农作物间作模式,评估其生产和经济效益,优化选择出了板栗与茶复合林模式、纯梨园、纯茶园、纯桃园等4种开发营林模式;板栗与山芋 雪菜、板栗与芝麻 胡罗卜、板栗与花生 苕子等3种板栗与农作物间模式。其中板栗与茶,并期板栗与山芋 雪菜等间作模式,可形成高效复合经营开发模式。文内还提出了该市低丘岗地综合治理与开发试点试区的建设原则,发展模式及应实施的集约组装技术。 相似文献