Validating the Use of 137Cs Measurements to Derive the Slope Component of the Sediment Budget of a Small Rangeland Catchment in Southern Italy

The sediment budget is a key concept and tool for characterizing the mobilization, transfer and storage of fine sediment within a catchment. Caesium‐137 measurements can provide valuable information on gross and net erosion rates associated with sheet and rill erosion that can be used to establish the slope component of a catchment sediment budget. However, there is a need to validate the use of ¹³⁷Cs measurements for this purpose, because their reliability has sometimes been questioned. The study reported focuses on a small (3·04 ha) steepland (mean slope 37%) catchment in Southern Italy. It exploits the availability of information on the medium‐term sediment output from the catchment provided by the construction of a reservoir at its outlet in 1978 and the existence of estimates of soil redistribution rates derived from ¹³⁷Cs measurements made on 68 replicate soil cores collected from the slopes of a substantial proportion of the catchment in 2001, to validate the use of ¹³⁷Cs measurements to construct the slope component of the catchment sediment budget. An additional 50 replicate soil cores were collected from the catchment slopes for ¹³⁷Cs analysis, to complement the data already available. Nine cores collected from the area occupied by the reservoir were used to estimate the mean annual sediment input to the reservoir. In the absence of evidence that the poorly developed channel system in the catchment was either a significant sediment source or sink, it was possible to directly compare the estimate of net soil loss from the catchment slopes (7·33 Mg ha⁻¹ y⁻¹) with the estimate of sediment output from the catchment provided by the reservoir deposits (7·52 Mg ha⁻¹ y⁻¹). Taking account of the uncertainties involved, the close agreement of the two values is seen as providing a convincing validation of the use of ¹³⁷Cs measurements to both estimate soil redistribution rates and as a basis for constructing the slope component of the sediment budget of a small catchment. Copyright © 2015 John Wiley & Sons, Ltd.     

Migration path and isotope tracing of 137Cs and 239 + 240Pu in estuary sediments: a case study of Liao River estuary in China

Purpose

Currently, the distribution characteristics and transport processes of the radionuclides ¹³⁷Cs and ^239?+?240Pu in the sediments of estuaries are still a controversial issue. Thus, in the present study, we investigated the distribution characteristics, sources and migration path of ¹³⁷Cs and ^239?+?240Pu in sediment cores of the Liao River estuary (LRE), China, and evaluated the relative contributions of the Pacific Proving Grounds (PPG) and riverine sources of Pu for the sediments in this area. We used ¹³⁷Cs and Pu isotopes for dating the sediments and estimated the sedimentation rates by the two radionuclides in the LRE.

Materials and methods

Seven sediment samples were collected using a box corer from the Liao River estuarine wetland and tidal flat in the LRE in October 2012 and April 2015, respectively. The activities of ¹³⁷Cs in the various samples were determined by γ spectrometry using HP-Ge detectors with 60% relative counting efficiency. Approximately 2–5 g of sediment were spiked with ²⁴²Pu (ca. 1 mBq) as a chemical yield tracer for Pu isotopic analysis at the School of Radiation Medicine and Protection, Soochow University. The measurement of Pu isotopes (²³⁹Pu, ²⁴⁰Pu, ²⁴²Pu) was performed by a sector field ICP-MS. In order to quantitatively differentiate the relative proportions of global fallout and PPG, we employed a two-end member mixing model to estimate their contributions.

Results and discussion

The average values of ¹³⁷Cs, ^239?+?240Pu activity concentrations, and ²⁴⁰Pu/²³⁹Pu atom ratios in the surface sediment samples of the LRE were 6.727?±?0.251 mBq g^?1, 0.294?±?0.024 mBq g^?1, and 0.188?±?0.049 (1σ), respectively. The average ²⁴⁰Pu/²³⁹Pu atom ratios ranged from 0.180?±?0.034 to 0.199?±?0.021 in sediment cores from the east and west sides of the LRE. For core LT-2 values for ¹³⁷Cs and ^239?+?240Pu concentrations were from below the detection limit: 3.380?±?0.414 and 0.036?±?0.007 to 0.105?±?0.007 mBq g^?1. The mean ²⁴⁰Pu/²³⁹Pu atom ratio 0.217?±?0.050 (1σ) in sediment core LT-2 lies between the global fallout and PPG close-in fallout.

Conclusions

We found that atmospheric fallout is the main source of Pu in sediment cores from the east and west sides of the LRE. For core LT-2, atmospheric fallout and riverine input (~?73.4%) are the major sources of Pu with the source of the rest of Pu (~?26.6%) attributed to the PPG via the Tsushima Warm Current and the coastal water of the East China Sea. The sedimentation rates (means 0.62–0.8 cm year^?1) estimated by the two radionuclides were in good agreement and without any statistically significant difference.

     

210Pb geochronology of sediment accumulation rates in Mexico City Metropolitan Zone as recorded at Espejo de los Lirios lake sediments

A sedimentary sequence from the Espejo de los Lirios lake in the Metropolitan Zone of Mexico City (MZMC) was analyzed in detail for ²¹⁰Pb and ¹³⁷Cs activities, allowing to assess the evolution of the accretion rates in the lake during the last ∼84±4 years. The core revealed the deposition of contemporaneously indigenous lake sediments to the site interspersed with eroded bedrock from the catchment, evidencing episodic increases in sediment accretion which varied from 0.14 to 0.93 cm year⁻¹. Increasing trends in sedimentation rates were found to be closely related to demographic expansion of the Metropolitan Zone of Mexico City and explained on the basis of the erosive processes produced as a result of deforestation created as a consequence of the urban and industrial development of the MZMC.     

Novel sediment source fingerprinting quantifying erosion-induced total nitrogen and total phosphorus outputs from an intensive agricultural catchment,North China

Intensive farming is a primary cause of increased sediment and associated nitrogen (N) and phosphorus (P) loads in surface water systems. Determining their contributing sources, pathways and loads present major challenges in the high-intensity agricultural catchments. Herein, we quantify the sediment sources and magnitude of sediment total N and total P from different sources using a novel application of compound-specific stable isotope (CSSI) and fallout radionuclides (FRNs) of ¹³⁷Cs and ²¹⁰Pbex in an intensive agricultural catchment in North China. Sediment sources from surface and sub-surface soils were estimated from FRNs fingerprint and accounted for 62 ± 7% and 38 ± 7% respectively, while surface soil from land uses that originated from hillslope were identified by CSSI fingerprint. Using a novel application of FRNs and CSSI sediment fingerprinting techniques, the dominant sediment source was derived from maize farmland (44 ± 0.1%), followed by channel bank (38 ± 7%). The sedimentation rate (13.55 ± 0.30 t ha⁻¹ yr⁻¹) was quantified by the ¹³⁷Cs cores (0–60 cm) at the outlet of this catchment. The total N and total P in sediment were both mostly derived from maize farmland and least from channel banks. The channel banks are significant sediment sources but contribute little to the input of sediment N and P for eutrophication. It implies that chemically-applied farmlands are the main hotspots for catchment erosion control and pollution prevention. The novel application of FRNs and CSSI techniques cost-effectively quantified sediment N and P loads from different sources with a single visit to the catchment, enabling rapid assessment for optimizing soil conservation strategies and land management practices. Keywords: Sediment sources, Land use, N and P loads, Compound-specific stable isotope, Fallout radionuclides.     

USE OF RESERVOIR DEPOSITS AND CAESIUM-137 MEASUREMENTS TO INVESTIGATE THE EROSIONAL RESPONSE OF A SMALL DRAINAGE BASIN IN THE ROLLING LOESS PLATEAU REGION OF CHINA

This paper reports the results of an investigation of the erosional response of the 3·86 km² Zhaojia Gully catchment in the rolling loess plateau region of Zichan County, Shaanxi Province, China. In the absence of direct measurements, information derived from reservoir deposits and from caesium-137 measurements on both the catchment soils and reservoir deposits was used to obtain a retrospective assessment of the longer-term (ca. 30 year) erosional response of the catchment and of the relative contributions of the rolling plateau surface and the gully areas to the sediment output from the basin. Net erosion rates on cultivated land occupying the gentle crest slopes and steeper lower slopes of the rolling plateau and the steep gully slopes were estimated to be 4500 t km⁻² year⁻¹, 8584 t km⁻² year⁻¹ and 15851 t km⁻² year⁻¹, respectively. Estimates of annual sediment yield from the study catchment based on analysis of sediment deposits in the two sediment-trap reservoirs ranged between 4627 and 32472 t km⁻² year⁻¹. Almost all the sediment transported from the catchment was contributed by 2–4 large floods each year. Measurements of the caesium-137 content of recent sediment deposits in a sediment-trap reservoir allowed the relative contributions of the total sediment yield derived from the rolling plateau and gully areas of the catchment to be estimated at 23 and 77 per cent, respectively. Analysis of the sediment deposits dating from 1973–1977 in another sediment trap reservoir allowed individual flood event couplets to be identified and indicated that the sediment associated with the first one or two floods in a season, when the soils of the plateau area were relatively dry, was derived primarily from the gully areas. The cultivated soils of the rolling plateau contributed an increased proportion of the total sediment yield during the latter stages of the flood season when the soils were wetter, and surface runoff and erosion were more widespread. Based on analysis of the caesium-137 content of the sediment deposited in this sediment-trap reservoir, the relative contributions of sediment from the rolling plateau and gully areas over the period 1973–1977 were estimated to be 21 and 79 per cent, respectively. The results obtained demonstrate the potential for using caesium-137 measurements and analysis of reservoir deposits to document the erosional response of a drainage basin. © 1997 John Wiley & Sons, Ltd.     

Establishing sediment budgets for two small lowland agricultural catchments in the UK

Sediment budgets have been established for two small (<4 km²), lowland, agricultural catchments, by using ¹³⁷Cs measurements, sediment source fingerprinting and more traditional monitoring techniques to quantify the individual components of the budget. The gross and net erosion rates for the fields on the catchment slopes were estimated using ¹³⁷Cs measurements within selected fields, which encompassed a representative range of slope angles, slope lengths and land use. These estimates were extrapolated over the entire catchment, using a simple topographically driven soil erosion model (Terrain-Based GIS, TBGIS) superimposed on a DEM, to derive catchment average gross and net erosion rates. Suspended sediment yields were measured at the catchment outlets and sediment source fingerprinting techniques were used to establish the relative contributions from the catchment surface, subsurface tile drains and eroding channel banks to the sediment yields. In-channel and wetland storage were quantified using both direct measurements and ¹³⁷Cs measurements. The sediment budgets established for the catchments highlighted the importance of subsurface tile drains as a pathway for sediment transfer, accounting for ca. 60% and 30% of the sediment output from the two catchments. Erosion from channel banks contributed ca. 10% and 6% of the sediment output from the two catchments. Although the suspended sediment yields from these catchments were considered high by UK standards (ca. 90 t km⁻² year⁻¹), the sediment delivery ratios ranged between 14% and 27%, indicating that a major proportion of the mobilised sediment was stored within the catchments. In-field and field-to-channel storage were shown to be of similar magnitude, but storage of sediment in the channel system and associated wetlands was relatively small, representing <5% of the annual suspended sediment yield.     

Simultaneous Use of Trace Metals, 210Pb and 137Cs in Floodplain Sediments of a Lowland River as Indicators of Anthropogenic Impacts

This study focuses on the distribution of selected trace metals, ¹³⁷Cs and ²¹⁰Pb, in floodplain deposits of the lowland Warta River (southern Poland) downstream of Cz?stochowa, a large city with an iron smelter. The depth profiles of trace metal (Zn, Pb, Cu, Ni, Cd and Mn), ²¹⁰Pb and ¹³⁷Cs contents in floodplain sediments were used to derive deposition rates on the floodplain for the twentieth century. The applicability of particular chronometric tools is considered within the context of their mutual relationships and confirmed by the consistency of the results. Deposition rate estimates for the past 50 years based on the vertical patterns of trace metal concentrations, which were correlated with particular events in the development of the smelter, range from 0.4 cm·year^?1 in profiles situated in backswamps far from the channel to over 1.1 cm·year^?1 in profiles of the natural levee adjacent to the river. Deposition rates based on ²¹⁰Pb inventories in the profiles range from 0.08 to 0.66 g·cm^?2·year^?1, which corresponds to linear sedimentation rates of 0.10 to 0.91 cm·year^?1, respectively. Dating of characteristic levels associated with peak fallout of ¹³⁷Cs gives sediment accretion rates resembling those obtained from trace metals and ²¹⁰Pb. The period of the highest sediment accumulation rate could be related to the highest loads of effluent from the iron smelter and city of Cz?stochowa, which were substantially reduced after the construction of effluent treatment plant.     

Mobilization of cesium in organic rich soils: Correlation with production of dissolved organic carbon

A study of the downward movement of ¹³⁷Cs in an undisturbed forest soil is presented. Seasonal variations and depth profiles of ¹³⁷Cs activities were measured in seepage water, which is the transport medium for the downward movement of anthropogenic substances in soils. Furthermore the correlation of ¹³⁷Cs mobilization and production of dissolved organic carbon (DOC) was investigated. Seasonal variations of both ¹³⁷Cs and DOC fluxes in the seepage water in a depth of 5 cm depth were observed, where the maximum fluxes in the summer months were about one order of magnitude higher than the minimum fluxes in the winter months. ¹³⁷Cs fluxes are found to be correlated with DOC fluxes with a correlation coefficient of r = 0.63, and both are highly correlated with soil temperature. This indicates that cesium is bound to soil organic material. The production of DOC is controlled by microbial decomposition of soil organic matter and we assume that this holds true for the ¹³⁷Cs release as well. The actual transport velocity (0.2 ± 0.14 mm/a) of ¹³⁷Cs (calculated by the weighed mean of ¹³⁷Cs concentration in the seepage water and the total ¹³⁷Cs content of the soil) is about one order of magnitude less than the mean transport velocity (1.2 ± 0.3 mm/a) over the past 25 years (calculated from the ¹³⁷Cs depth profile). It is possible that the transport velocity of ¹³⁷Cs in undisturbed soils decreases with time as it binds to aged organic material which is less easily decomposable than fresh organic material.     

Distribution of 137Cs and 60Co in plough layer of farmland: Evidenced from a lysimeter experiment using undisturbed soil columns

Radionuclide fallout during nuclear accidents on the land may impair the atmosphere, contaminate farmland soils and crops, and can even reach the groundwater. Previous research focused on the field distribution of deposited radionuclides in farmland soils, but details of the amounts of radionuclides in the plough layer and the changes in their proportional distribution in the soil profile with time are still inadequate. In this study, a lysimeter experiment was conducted to determine the vertical migration of 137Cs and 60Co in brown and aeolian sandy soils, collected from the farmlands adjoining Shidaowan Nuclear Power Plant(NPP) in eastern China, and to identify the factors influencing their migration depths in soil. At the end of the experiment(800 d), >96% of added 137Cs and 60Co were retained in the top 0–20 cm soil layer of both soils;very little 137Cs or 60Co initially migrated to 20–30 cm, but their amounts at this depth increased with time. The migration depth of 137Cs was greater in the aeolian sandy soil than in the brown soil during 0–577 d, but at the end of the experiment, 137Cs migrated to the same depth(25 cm) in both soils. Three phases on the vertical migration rate(v) of 60Co in the aeolian sandy soil can be identified: an initial rapid movement(0–355 d, v = 219 ± 17 mm year-1), followed by a steady movement(355–577 d, v = 150 ± 24 mm year-1) and a very slow movement(577–800 d, v = 107 ± 7 mm year-1). In contrast, its migration rate in the brown soil(v = 133 ± 17 mm year-1) was steady throughout the 800-d experimental period. The migration of both 137Cs and 60Co in the two soils appears to be regulated by soil clay and silt fractions that provide most of the soil surface area, soil organic carbon(SOC), and soil pH, which were manifested by the solid-liquid distribution coefficient of 137Cs and 60Co. The results of this study suggest that most 137Cs and 60Co remained within the top layer(0–20 cm depth) of farmland soils following a simulated NPP accident, and little reached the subsurface(20–30 cm depth). Fixation of radionuclides onto clay minerals may limit their migration in soil, but some could be laterally distributed by soil erosion and taken up by crops, and migrate into groundwater in a high water table level area after several decades.Remediation measures, therefore, should focus on reducing their impact on the farmland soils, crops, and water.     

Relating Intensity of Soil Redistribution to Land Use Changes in Abandoned Pyrenean Fields Using Fallout Caesium‐137

Fallout caesium‐137 has been used to trace soil redistribution in abandoned fields located in the Central Spanish Pyrenees. A total of 28 fields with different lengths, slope angles and time since abandonment were selected on a representative south‐facing slope of the Estarrún valley. The local reference inventory and the magnitude and spatial distribution of ¹³⁷Cs inventories within these fields were documented and used as a basis for assessing patterns of soil redistribution. The local reference inventory was estimated to be 4,500 Bqm⁻². Within the fields, the average ¹³⁷Cs inventory at the top of the slope was 3,920 Bqm⁻², and accumulation of soil at the bottom of the slopes was demonstrated by an average ¹³⁷Cs inventory of 5,320 Bqm⁻². Deviations from the reference inventory were highest for fields with the longest slopes that had been abandoned for less than 30 years. Here, increases in the ¹³⁷Cs inventory, relative to the reference inventory, in excess of 20% were found at the bottom of the slopes. Considering all the fields and all geomorphic positions within the fields, the greatest ¹³⁷Cs losses and gains were found in the fields with the longest duration of abandonment, indicating more intense soil redistribution. Irrespective of the timing of abandonment, the ranges of ¹³⁷Cs inventories in the fields were found to be proportional to the water erosion index. The ¹³⁷Cs technique demonstrated that patterns of sediment redistribution were closely related to the topographic and physiographic characteristics of the slopes. Copyright © 2017 John Wiley & Sons, Ltd.     

桑干河流域淤地坝沉积泥沙特征及其来源解析

[目的]为查明桑干河流域的泥沙主要策源地和侵蚀产沙变化。[方法]选取阳原县高墙乡典型淤地坝沉积泥沙为研究对象,利用复合指纹识别技术,测定沉积泥沙及其源地的土壤粒径、SOC、TN、¹³⁷Cs、低频质量磁化率等9种指纹因子,研究了不同淤积阶段的泥沙策源地及坝控小流域侵蚀产沙演变规律。[结果](1)沉积泥沙中¹³⁷Cs平均含量较低,与沟壁土壤无显著差异(p>0.05),但极显著小于林草地和耕地的¹³⁷Cs含量(p<0.01),这指示淤地坝沉积泥沙主要来源于沟壁;(2)由于沟壁中大部分¹³⁷Cs含量低于检出限,¹³⁷Cs较好地指示泥沙主要来源沟谷地中的沟壁,但难以用于小流域多种策源地的判别,经Kruskal-Wallis H非参数检验和多元逐步判别分析筛选,确定TN+X_lfb+SOC构成最佳指纹因子组合,有效地判别小流域2006—2017年泥沙源地的平均贡献率为沟壁(82.68%±8.20%)>耕地(15.36%±8.46%)>林草地(1....     

Recent sedimentation rates in Garaet El Ichkeul Lake, NW Tunisia, as affected by the construction of dams and a regulatory sluice

Purpose

Ichkeul National Park, NW Tunisia, is a UNESCO Biosphere Reserve. Garaet El Ichkeul Lake is known for its seasonal variability in water level and salinity. In recent decades, the waterbody has been affected by the construction of new hydraulic structures. To reduce the impacts of dams and to maintain the sustainability of the ecosystem, a sluice was built at the outlet of the lake, and it operated for the first time in 1996. This paper describes an investigation of recent sedimentation dynamics in Ichkeul Lake, determined by radiometric dating of sediment cores.

Materials and methods

A sediment core was collected with a UWITEC gravity corer at the deepest, central part of the lake in August 2009. Specific activities of unsupported lead-210 (²¹⁰Pb) and caesium-137 (¹³⁷Cs) were measured in the core, enabling calculation of recent sediment accumulation rates (SAR). Published radiometric data from nearby sediment cores, collected in 1997 and 1982, provide a comparison.

Results and discussion

The measured excess ²¹⁰Pb inventory was 5300?±?500?Bq?m^?2, leading to an estimation of constant flux of 165?±?16?Bq?m^?2?yr^?1, a value higher than the best estimate for local atmospheric fluxes (123?±?12?Bq?m^?2?yr^?1) and the flux estimated from the core collected in 1982 (48?Bq?m^?2?yr^?1). The ¹³⁷Cs inventory was 3550?±?120?Bq?m^?2, two times higher than the historical ¹³⁷Cs atmospheric deposition in the area. The ¹³⁷Cs profile displayed a distinct peak, but the ¹³⁷Cs depth-distribution did not follow the pattern expected from atmospheric deposition. Application of the constant rate of supply (CRS) model, with the reference point method, produced a chronology and SAR values comparable to those found in previous work. The whole ¹³⁷Cs profile was quantitatively reconstructed from the historical records of atmospheric deposition, using the system-time-averaged (STA) model.

Conclusions

The CRS and STA models provide consistent sediment accumulation results for the whole data set, considering the time resolution of the chronology (~6?years) and analytical uncertainties. Results from cores sampled in 1982, 1997 and 2009 reveal an increasing SAR trend, from ~0.25?g?cm^?2?yr^?1 in the early 1940s to ~0.67?g?cm^?2?yr^?1 at present. In the 13?years since installation of sluice gates at Tinja, SAR in the central Ichkeul Lake has not declined. Thus, if siltation continues at the present rate, shallowing of the lake will seriously affect the hydromorphology and ecology of this important lake.     

Integrated assessment of catchment suspended sediment budgets: a Zambian example

In many developing countries, the management of sediment‐related environmental problems is severely hampered by a lack of information on sediment mobilization and delivery in river basins. The sediment budget concept represents a valuable framework for assembling such information, which can, in turn, be used to assist with the design and implementation of soil erosion and sediment control policies. However, the information necessary to construct a catchment sediment budget is difficult to assemble. Against this background, an integrated approach to establishing a catchment suspended sediment budget, involving a river monitoring station, the use of ¹³⁷Cs measurements to estimate soil erosion and deposition and floodplain accumulation rates within the catchment, and sediment source fingerprinting, has been developed and tested in the 63 km² catchment of the upper Kaleya River in southern Zambia. The approach developed not only provides detailed information on individual components of the suspended sediment delivery system, but also permits the establishment of the overall catchment sediment budget. A sediment budget for the upper Kaleya catchment is presented and both its key features and its wider implications for catchment management are discussed. Copyright © 2001 John Wiley & Sons, Ltd.     

Quantification of accelerated soil erosion using the environmental tracer caesium-137

The principal objective of this investigation was to quantify erosion rates for five agricultural fields in three separate study areas in Saskatchewan. The radionuclide tracer caesium-137 (¹³⁷Cs) was used to quantify net erosion and net deposition within the landscape over a 30-year period. Uneroded (native) sites were used to establish the mean background level of ¹³⁷Cs in each of the study areas. The assumption being that agricultural sites with ¹³⁷Cs areal activities greater than the native site were subject to deposition, and sites with ¹³⁷Cs less than the native control site were subject to erosion. A linear proportionality model was used to convert the loss or gain of ¹³⁷Cs to net soil erosion or deposition. Results have indicated that accelerated (anthropogenic) erosion has been commonplace on arable land in Saskatchewan, even on near-level fields (< 1.3 degrees). The net integrated sediment output from the five agricultural fields ranged from — 0.6 t th⁻¹ y⁻¹ to — 6.8 t ha⁻¹ y⁻¹ (where negative values represent erosion). What is more alarming is that between 40 and 75 per cent of all sites sampled within individual fields had erosion rates in excess of the generally accepted rate of soil formation (1.0 t ha⁻¹ y⁻¹). Also, in one highly eroded field (Crystal Springs medium sloping site) 65 per cent of the sites sampled exceeded the upper tolerable erosion rate of 11.0 t ha⁻¹ y⁻¹. These results indicate significant degradation of the non-renewable soil resource has occurred over the past 30 years and is still presently active. Land degradation by accelerated erosion would result in reductions in effective rooting depth, soil moisture holding capacity, essential nutrient stores, and would adversely effect the physical structure of the topsoil. The major reason for accelerated erosion on arable land in Saskatchewan is the practice of summer fallowing, where the field is left in a ‘bare’ state and repeatedly tilled every second or third year. During a fallow period, or prior to crop emergence during a cropping year, fields are subject to wind and water erosion. On near-level fields wind would be the dominant transport agent, while on sloping fields inter-rill and rill erosion would be the primary forces of erosion. It is suggested that the appropriate conservation farming response would be to increase application of surface mulches and possibly to decrease the frequency of summer fallowing. Without such efforts long-term sustainable agricultural production in the Prairies of Canada is considered to be a tenuous land use practice.     

Transfer of 137Cs and 40K from Agricultural Soils to Food Products in Terrestrial Environment of Tarapur, India

The ¹³⁷Cs and ⁴⁰K activities and transfer factors from soil to vegetables, grass, and milk from villages located around Tarapur Atomic Power Station (TAPS) were determined using high-resolution gamma spectrometry. A total of 32 soil, 21 vegetable, 23 dry paddy grass, and 23 milk samples were collected from 23 different agricultural farms from various villages around TAPS to determine transfer factors for natural environment. The mean concentration values for ¹³⁷Cs and ⁴⁰K in soil, grass, and milk were 2.39?±?0.86 Bq kg^?1, 0.31?±?0.23 Bq kg^?1, and 12.4?±?5.7 mBq L^?1 and 179?±?31 Bq kg^?1, 412?±?138 Bq kg^?1, and 37.6?±?9.3 Bq L^?1, respectively, for soil?Cgrass?Cmilk pathway. In the soil?Cvegetation pathway, the mean concentrations values for ¹³⁷Cs and ⁴⁰K were 2.15?±?1.04 Bq kg^?1, 16.5?±?7.5 mBq kg^?1, and 185?±?24, 89?±?50 Bq kg^?1, respectively. The evaluated mean transfer factors from soil?Cgrass, grass?Cmilk, and soil?Cvegetation for ¹³⁷Cs were 0.14, 0.0044, and 0.0073 and that of ⁴⁰K were 2.42, 0.0053, and 0.49, respectively. Only 15 out of total 44 milk and vegetable samples were detected positive for ¹³⁷Cs, indicating a very low level of bioavailability.     

Distribution of <Superscript>137</Superscript>Cs in the particle-size fractions and in the profiles of alluvial soils on floodplains of the Iput and its tributary Buldynka Rivers (Bryansk oblast)

Pits of sandy alluvial soils were studied in different parts of the floodplains of the Iput River and its tributary the Buldynka River near the settlement of Starye Bobovichi (Bryansk oblast). The ¹³⁷Cs content in the soil horizons varied from 0.01 to 31.2 Bq/g reaching the maximum in the initially polluted layers buried at depths of 6 to 40 cm. Radiocesium was found in all the particle-size fractions with its predominate concentration in the finest fractions. The specific ¹³⁷Cs activity in the fractions of <1, 1–5, 5–10, and >10 μm comprised 44.1 ± 11.5; 33.3 ± 7.6, 20.9 ± 4.9, and 2.4 ± 0.6 Bq/g of soil. However, the contribution of the coarse (>10 μm) fractions to the total radiocesium pool in the soils (19–60%, or 34 ± 2% on the average) was comparable with that of the clay fraction (16–71%, or 38 ± 3% on the average), because of the predominance of the sand-size fractions in the soils. The highest coefficient of variation with respect to the relative contribution of particular fractions to the total soil pool of ¹³⁷Cs was characteristic of the fraction of 5–10 μm; in the other fractions, it varied from 31 to 41%. The portion of ¹³⁷Cs bound with the finest fractions increased in the deeper layers. The total ¹³⁷Cs activity in the polluted horizons of the soils was mainly determined by its concentration in the clay fraction (Spearman’s coefficient of rank correlation (r) for the moderately polluted horizons comprised 0.926 at n = 14). It was experimentally proved that clay particles, upon the destruction of organic films on their surface, could readsorb the released radiocesium for a second time.     

Caesium-137 fallout depth distribution in different soil profiles and significance for estimating soil erosion rate

Caesium-137 (¹³⁷Cs) has been widely used for the determination of soil erosion and sediment transport rate. However, depth distribution patterns of ¹³⁷Cs in the soil profile have not been considered. As a result, the erosion rates may be over-estimated or underestimated. This paper presents the depth distribution of ¹³⁷Cs fallout in different soil profiles using published data. Three types of depth distribution functions of ¹³⁷Cs are given by using statistical regression methods, the exponential type, the peak type and the decreasing type (including uniform distribution). Relationships between ¹³⁷Cs loss and soil erosion rate are given by introducing the regression functions. The influence of depth distribution of ¹³⁷Cs on the estimation of the soil erosion rate was simulated. Simulation results showed that very different soil erosion rates could be deduced for different depth distributions when ¹³⁷Cs loss is the same, which indicates that the depth distribution pattern should be considered when soil erosion is estimated by using ¹³⁷Cs. Simulation results also suggested that it is most important to determine the depth distribution of ¹³⁷Cs near the soil surface and the annual relative loss of ¹³⁷Cs by using the depth distribution of ¹³⁷Cs as a criterion to estimate the soil erosion rate.     

Investigating the effects of afforestation on soil erosion and sediment mobilisation in two small catchments in Southern Italy

Annual soil losses in southern Italy can exceed 100–150 t ha^− 1 year^− 1. Where erosion on agricultural land is particularly severe, land use change and afforestation are frequently seen as the most appropriate means of reducing erosion risk. However, the overall effectiveness of afforestation in reducing soil erosion remains uncertain, due to the poor development of the forest cover in some areas, leading to significant areas with sparse tree cover, and the erosional impact of forest harvesting, which commonly involves clearcutting. The study reported here addresses this uncertainty and focuses on two small catchments (W2 and W3) located in Calabria, southern Italy, for which measurements of suspended sediment yield are available. Both the catchments originally supported a rangeland vegetation cover and they were planted with eucalyptus trees in 1968. Currently, only catchment W3 supports a continuous forest cover. In catchment W2 the forest cover is discontinuous and there is a significant area of the catchment (ca. 20%) where the tree cover is sparse and the vegetation cover is dominated by natural grasses. Two additional erosion plots were established within catchment W2 in 1991, in order to explore the effect of the density of the tree cover on soil erosion. Information on the sediment yields from the two catchments and the plots for 10 storm events that occurred during the period December 2005–December 2006 and associated information on the ¹³⁷Cs and excess ²¹⁰Pb of the sediment, have been used to investigate the effectiveness of afforestation in reducing sediment mobilisation and net soil loss from the catchments involved. The results demonstrate that the areas of greatest soil loss are associated with the slopes where the tree cover is discontinuous, and that forest harvesting by clearcutting causes significant short-term increases in sediment mobilisation and sediment yield. These findings, which are consistent with previous work undertaken within the same area, emphasize the importance of vegetation cover density in influencing rates of soil loss in the study catchments. The study also provided a useful demonstration of the potential for using measurements of the ¹³⁷Cs and ²¹⁰Pb_ex content of sediment, in combination with more traditional sediment monitoring, to investigate sediment sources and to compare the sediment dynamics of catchments subjected to different land management practices.     

Use of fallout Cs in investigations of overbank sediment deposition on river floodplains

River floodplains have been recognised as important sinks for storing suspended sediment and associated contaminants mobilised from the upstream catchment. However, information on contemporary rates of overbank sedimentation is difficult to obtain using conventional methods. Measurements of the ¹³⁷Cs content of floodplain sediments provide an alternative approach to obtaining; estimates of medium-term rates (ca. 40 years) of overbank sediment deposition. The ¹³⁷Cs approach requires only a single site visit and minimum sample preparation. Furthermore, it is capable of providing information on spatial patterns of sediment deposition on floodplains, which is needed to improve our understanding of the processes involved in overbank flow and sediment deposition. This paper reviews the basis for using ¹³⁷Cs measurements in floodplain sedimentation studies and presents improved procedures for interpreting ¹³⁷Cs profiles in floodplain sediments and for obtaining estimates of sedimentation rates from single measurements of the total. ¹³⁷Cs inventories of bulk sediment cores. The results obtained from a case study undertaken on the floodplain of the River Stour, Dorset, UK, are presented.     

Using Cs‐137 fingerprinting technique to estimate sediment deposition and erosion rates from Yongkang depression in the karst region of Southwest China

Understanding the erosion and deposition rates is very important for designing soil and water conservation measures. However, existing methods of assessing the rates of soil loss present many limitations and are difficult to apply to in karst areas, and there is still very little data in this areas. Karst depressions comprise geomorphologically important sources and sinks for sediments and can provide the long‐term history records of environmental changes. But there have been few similar studies focused on its sediments in the world. In this paper, the Cs‐137 technique was employed to estimate the sediment deposition rate of karst depression to assess the surface erosion. The results indicate that the average deposition rate, deposition amount and specific deposit yield for the Yongkang catchments since 1963 were estimated to be 4·32 mm y⁻¹, 3·16 t y⁻¹and 20·53 t km⁻² y⁻¹, respectively. The results obtained were consistent with the actual monitoring data of local runoff plots, and confirm the validity of the overall approach. So it was suggested that the mean specific sediment yields of 20 t km⁻² y⁻¹ can be representative of the soil loss rates in the regions. Copyright © 2010 John Wiley & Sons, Ltd.