Transfer of radiocesium from hydroponic medium to potherb mustard and tomato plants

Abstract

Potherb mustard (Brassica rapa var. nipposinica) and tomato plants (scion, ‘CF Momotaro haruka’; rootstock, ‘Dokutar K’; Solanum lycopersicum) were cultured in hydroponic medium containing cesium-137 (¹³⁷Cs) at three different concentrations (0.03, 0.13 and 1.03 Bq L^?1), and uptake of ¹³⁷C into the plants was determined. When the ¹³⁷Cs radioactivity concentration in the medium was 1.03 Bq L^?1, the ¹³⁷Cs radioactivity concentrations in the edible portions of the plants were 4.80 Bq kg^?1 fresh weight for the potherb mustard plants and 3.60 Bq kg^?1 fresh weight for the tomato plants. In both species, the ¹³⁷Cs radioactivity concentration in the edible portions decreased with decreasing ¹³⁷Cs radioactivity concentration in the culture medium. When the ¹³⁷Cs radioactivity concentration in the medium was 0.03 Bq L^?1, a concentration observed in many streams and in tap water in Fukushima Prefecture after the accident at the Fukushima Daiichi Nuclear Power Plant, the ¹³⁷Cs radioactivity concentrations in the edible portions of the plants were 0.50 and 0.15 Bq kg^?1 fresh weight for potherb mustard and tomato plants, respectively. These values are less than the Japanese allowable limit for radiocesium in food. For both species, the transfer factors for ¹³⁷Cs uptake from the culture media to the edible portions and the average transfer rates over the cultivation period were calculated.     

West Valley-derived radionuclides in the Niagara river area of Lake Ontario

The presence of West Valley-derived radionuclides in the densely-populated Niagara River/Lake Ontario region is demonstrated through measurements on water and sediment samples. The ¹³⁷Cs profile in a ²¹⁰Pb-dated Lake Ontario sediment core is consistent with the pattern of West Valley discharges to the local aquatic environment in that the observed ¹³⁷Cs activity maximum corresponds to the 1970 peak discharge and not the 1963 fallout peak activity. Preliminary mass balance estimate, based on a ¹³⁷Cs/⁹⁰Sr activity ratio of 1.5 and on the assumption that the dominant regional flow of Lake Erie transports most of the radionuclides to Lake Ontario va the Niagara River, shows that nearly all of the West Valley-delivered ¹³⁷Cs is deposited in the bottom sediments of Lake Ontario. It is suggested that any accidental releases of radioactivity from the site are likely to provide additional radiation dose to the area residents using municipal water supplies.     

Quantification of accelerated soil erosion using the environmental tracer caesium-137

The principal objective of this investigation was to quantify erosion rates for five agricultural fields in three separate study areas in Saskatchewan. The radionuclide tracer caesium-137 (¹³⁷Cs) was used to quantify net erosion and net deposition within the landscape over a 30-year period. Uneroded (native) sites were used to establish the mean background level of ¹³⁷Cs in each of the study areas. The assumption being that agricultural sites with ¹³⁷Cs areal activities greater than the native site were subject to deposition, and sites with ¹³⁷Cs less than the native control site were subject to erosion. A linear proportionality model was used to convert the loss or gain of ¹³⁷Cs to net soil erosion or deposition. Results have indicated that accelerated (anthropogenic) erosion has been commonplace on arable land in Saskatchewan, even on near-level fields (< 1.3 degrees). The net integrated sediment output from the five agricultural fields ranged from — 0.6 t th⁻¹ y⁻¹ to — 6.8 t ha⁻¹ y⁻¹ (where negative values represent erosion). What is more alarming is that between 40 and 75 per cent of all sites sampled within individual fields had erosion rates in excess of the generally accepted rate of soil formation (1.0 t ha⁻¹ y⁻¹). Also, in one highly eroded field (Crystal Springs medium sloping site) 65 per cent of the sites sampled exceeded the upper tolerable erosion rate of 11.0 t ha⁻¹ y⁻¹. These results indicate significant degradation of the non-renewable soil resource has occurred over the past 30 years and is still presently active. Land degradation by accelerated erosion would result in reductions in effective rooting depth, soil moisture holding capacity, essential nutrient stores, and would adversely effect the physical structure of the topsoil. The major reason for accelerated erosion on arable land in Saskatchewan is the practice of summer fallowing, where the field is left in a ‘bare’ state and repeatedly tilled every second or third year. During a fallow period, or prior to crop emergence during a cropping year, fields are subject to wind and water erosion. On near-level fields wind would be the dominant transport agent, while on sloping fields inter-rill and rill erosion would be the primary forces of erosion. It is suggested that the appropriate conservation farming response would be to increase application of surface mulches and possibly to decrease the frequency of summer fallowing. Without such efforts long-term sustainable agricultural production in the Prairies of Canada is considered to be a tenuous land use practice.     

Radio-caesium fixation dynamics: measurement in six Cumbrian soils

Five peat soils and a mineral soil were artificially contaminated with ¹³⁷Cs. Soil solution activity and radio–lability of ¹³⁷Cs were monitored over 709 days to quantify progressive ¹³⁷Cs fixation. The peat soils fixed large amounts of ¹³⁷Cs, but less than the mineral soil did. Distribution coefficients (K_d, cm³ g^?1) ranged from 30 to 5000 at the end of equilibration. A labile ¹³⁷Cs distribution coefficient, K_dt, was estimated by a method involving solid ? solution equilibration in dilute solution. In a separate study several concentrations of KCl were added to soils in increasing concentration both before and after the addition of ¹³⁷Cs. Differences in apparent adsorption strength of radiocaesium indicated that K⁺ induced the collapse of expanded mineral interlayers, thereby trapping ions. It seemed that ^I37Cs adsorbs at sites in the small micaceous clay fraction of the peat soils. The different rates of ¹³⁷Cs adsorption and fixation in the peat and mineral soils, in which the rate of access of ¹³⁷Cs to fixation sites in peat soils is less, seems to have been caused partly by lack of K, and partly by the scarcity of fixation sites.     

Assessment of soil erosion on arable land using Cs measurements: a case study from Jaslovske Bohunice, Slovakia

This study was carried out to obtain a representative set of data on long-term erosion rates from a pilot area located close to the Jaslovske Bohunice village, in western Slovakia using the ¹³⁷Cs-method. The study area chosen was representative of the hilly loess cultivated areas of Slovakia. The sampling strategy was based on a multiple transect approach. Analyses of the samples for ¹³⁷Cs activity were made at the Nuclear Power Plant Research Institute, Jaslovske Bohunice. The ¹³⁷Cs-method was used to obtain long-term estimates of soil erosion in the Jaslovske Bohunice site, a representative hilly loess cultivated area of Slovakia. The estimated reference ¹³⁷Cs inventory was 2910 Bq m⁻², with a coefficient of variation of 4.3%.Examination of the ¹³⁷Cs redistribution in relation to the topography of the study area revealed that, within individual transects the ¹³⁷Cs inventories were closely related to major landforms. The ¹³⁷Cs inventories were considerably lower on the slopes than on the plateau and they were highest in the valley. However, when plotted against a selection of individual quantitative slope parameters, i.e. the S and the LS factors of the USLE or slope inclination, the correlations obtained were weak.Three conversion models, i.e. the proportional model (PM), the simplified mass balance model (MBM1) and the standard mass balance model (MBM2), from the set of models developed at Exeter University, Great Britain were selected to interpret the resulting ¹³⁷Cs measurements into soil erosion/deposition rates. The mean erosion rates estimated with the PM were 22.4, 35.6 with MBM1 and 17.3 t ha⁻¹ per year with MBM2. There was a good agreement between the average of these mean erosion rates (25.1 t ha⁻¹ per year) for the Jaslovske Bohunice site and the estimated mean soil erosion rate obtained for small erosion plots (15 t ha⁻¹ per year) for conditions similar to the study site. Nevertheless, further research on the application of the ¹³⁷Cs-method, in particular the independent validation of the results obtained, is needed. Several issues requiring further study have been highlighted.     

Radioactive cesium distribution in bamboo [Phyllostachys reticulata (Rupr) K. Koch] shoots after the TEPCO Fukushima Daiichi Nuclear Power Plant disaster

Abstract

Radioactivity levels of cesium (Cs)-134 and ¹³⁷Cs in bamboo [Phyllostachys reticulata (Rupr) K. Koch] sprouts grown from April to June 2011 over a wide area (including Fukushima Prefecture) were elevated (max. 3100 Bq kg^?1 fresh weight) after the Tokyo Electric Power Company, Inc. (TEPCO) Fukushima Daiichi Nuclear Power Plant disaster in March 2011. Bamboo sprouts in 2012 also contained high radioactivity levels. Radioactivity imaging analysis of bamboo sprouts harvested in 2012 showed increasing concentration gradients of radioactivity from the lower parts to the top of the sprouts. The peels were individually separated from the sprouts, and the inner edible part (trunk) was cross-sectioned at the internodal sections from the top to the lower parts. Each segmented trunk and its corresponding peel were analyzed for radioactive cesium (¹³⁴Cs and ¹³⁷Cs) and stable cesium (¹³³Cs). The concentrations of ¹³⁴Cs and ¹³⁷Cs showed significant increases from the lower part to the top, whereas ¹³³Cs showed an almost constant value in the trunk and peel except in the peel of the top node. We speculated that ¹³⁴Cs and ¹³⁷Cs in newly emerging bamboo sprouts in 2012 were translocated mainly from various plant tissues (where the fallout was layered on the bamboo tissues) in older bamboo, while ¹³³Cs was translocated from the soil through the roots of the new bamboo sprouts and was present in the roots and stems.     

Use of Cs to estimate tillage- and water-induced soil redistribution rates on agricultural land under different use and management in central-south Chile

The purpose of this research was to evaluate the applicability of conventional ¹³⁷Cs sampling and a simplified approach, for estimating medium-term tillage- and water-induced soil erosion and sedimentation rates on agricultural land in Chile. For this purpose, four study sites under contrasting land use and management were selected in central-south Chile. First, a conventional ¹³⁷Cs approach, based on grid sampling was applied, adapting a mass balance conversion model incorporating soil movement by tillage to the site specific conditions of the study region. Secondly, using the same conversion model, the feasibility of estimating soil redistribution rates from measurements of ¹³⁷Cs inventories based on composite soil samples taken along contour lines was also tested at all four sites. The redistribution rates associated with tillage and water and the total rates estimated using both methods correlated strongly at all four sites. The conventional method provides more detailed information concerning the redistribution processes operating over the landscape. The simplified method is suitable for assessing soil loss and sediment accumulation in areas exhibiting simple topography and almost similar slopes along the contour lines. Under these conditions, this method permits faster estimation of soil redistribution rates, providing the possibility of estimating soil redistribution rates over larger areas in a shorter time. In order to optimise the costs and benefits of the methods, the sampling and inventory quantification strategy must be selected according to the resolution of the required information, and the scale and complexity of the landscape relief. Higher tillage- and water-induced erosion rates were observed in the annually ploughed cropland sites than in the semi-permanent grassland sites. Subsistence managed crop and grassland sites also show greater erosion effects than the commercially managed sites. The ¹³⁷Cs methods used permit discrimination between redistribution rates observed on agricultural land under different land use and management. The ¹³⁷Cs technique must be seen as an efficient method for estimating medium-term soil redistribution rates, and for planning soil conservation and sustainable agricultural production under the climatic conditions and the soil type of the region of Chile investigated.     

利用137Cs示踪技术评价东北黑土侵蚀和沉积过程

Soil and water losses through erosion have been serious in the black soil region of Northeast China. Therefore, a sloping cultivated land in Songnen Plain was selected as a case study to： 1） determine the ^137Cs reference inventory in the study area; 2） calculate erosion and deposition rates of black soil on different slope locations; 3） conduct a sensitivity analysis of some model parameters; and 4） compare overall outputs using four different models. Three transects were set in the field with five slope locations for each transect, including summit, shoulder-slope, back-slope, foot-slope, and toe-slope. Field measurements and model simulation were used to estimate a bomb-derived ^137Cs reference inventory in the study area. Soil erosion and deposition rates were estimated using four ^137Cs models and percentage of ^137Cs loss/gain. The ^137Cs reference value in the study area was 2 232.8 Bq m^-2 with ^137Cs showing a clear topographic pattern, decreasing from the summit to shoulder-slope, then increasing again at the foot-slope and reaching a maximum at the toe-slope, Predicted soil redistribution rates for different slope locations varied. Among models, the Yang Model （YANG-M） overestimated erosion loss but underestimated deposition. However, the standard mass balance model （MBM1） gave predictions similar to a mass balance model incorporating soil movement by tillage （MBM2）. Sensitivity analysis of the proportion factor and distribution pattern of ^137Cs in the surface layer demonstrated the impact of ^137Cs enrichment on calculation of the soil erosion rate. Factors influencing the redistribution of fallout ^137Cs in landscape should be fully considered as calculating soil redistribution rate using ^137Cs technique.     

Accumulation of radioactive cesium in sorghum (Sorghum bicolor (L.) Moench) accessions cultivated in Fukushima in 2011 and 2012

ABSTRACT

The accident at Fukushima 1 Nuclear Power Plant in 2011 caused contamination by radioactive cesium (¹³⁴Cs and ¹³⁷Cs) in surrounding areas. After this accident, concerns about Cs contamination, including food safety, have limited industrial activities and reconstruction in Fukushima. Sorghum (Sorghum bicolor (L.) Moench) is an annual C₄ crop that can be used as biofuel feedstock due to its high biomass. Use of Cs-contaminated fields to produce biofuel feedstock would be more acceptable than use for food or feed crops due to the lower risk of human internal exposure to radioactive Cs. In addition, high-biomass sorghum might be suitable for removal of Cs from fields (phytoremediation). For both applications, it is important to use accessions showing the appropriate level of accumulation of radioactive Cs (low for biofuel feedstock, high for phytoremediation). Here, we examined the accumulation of radioactive Cs in the aerial parts of 56 sorghum accessions grown in Fukushima. Accessions were cultivated in a low-level-contaminated field in 2011 and in a highly contaminated field in a planned evacuation zone in 2012. After cultivation, activity concentrations from ¹³⁴Cs and ¹³⁷Cs were measured in the aerial plant parts. In 2011, the activity concentrations of ¹³⁴Cs and ¹³⁷Cs were 58.2–350 and 58.6–450 Bq kg^?1 dry weight, respectively. In 2012, the concentrations of ¹³⁴Cs and ¹³⁷Cs were 54.2–1320 and 57.1–1960 Bq kg^?1 dry weight, respectively. Relative to the median values of the accessions grown each year, 3 showed lower activity concentrations and 2 showed higher activity concentrations of radioactive Cs under both cultivation conditions. In contrast to a previous report, there was no significant correlation between biomass and Cs activity concentration. Because both biomass and Cs concentration are important in classifying accessions for use in phytoremediation, we also calculated the Cs accumulation index (single-plant biomass × Cs activity concentration) for each accession. The accession AKLMOI WHITE showed the highest values in both years, suggesting that this accession has the high per-plant accumulation capacity for radioactive Cs. Our data collected from actual contaminated fields is irreplaceable for choosing sorghum accessions for cultivation in Cs-polluted sites such as Fukushima.     

中国南方红壤地区的137Cs基准点的选取

The ^137Cs vertical distributions in uncultivated and cultivated soils, developed from Quaternary red clay, granite, argillaceous shale, and red sandstone, were studied to develop reliable guidelines for selecting reference sites in southeastern China, which is dominated by strong acidic and/or clay-textured soils, and examine their reliability by comparing them to the reported ^137Cs reference inventory data to see whether they agreed with the global distribution pattern. It was observed that a relatively high proportion of ^137Cs was concentrated in the surface layers of soils with relatively high clay content. In the paddy soils developed from granite more ^137Cs penetrated to depths below the plow layer （about 45.3%）, when compared to those from the other three parent materials. The relatively low soil ^137Cs inventories on crests excluded using the crest as the ^137Cs reference site; instead the paddy field on the hillock plain was selected. Furthermore, within a specific county characterized by great systematic spatial variations of rainfall and topography across the landscape, a significant （P 〈 0.01） and positive linear relationship （r^2 = 0.81） between local ^137Cs inventory and corresponding local annual rainfall was observed. Thus, for areas with large variations in rainfall, a single uniform value of local ^137Cs reference inventory should be used with caution.     

Use of fallout Cs in investigations of overbank sediment deposition on river floodplains

River floodplains have been recognised as important sinks for storing suspended sediment and associated contaminants mobilised from the upstream catchment. However, information on contemporary rates of overbank sedimentation is difficult to obtain using conventional methods. Measurements of the ¹³⁷Cs content of floodplain sediments provide an alternative approach to obtaining; estimates of medium-term rates (ca. 40 years) of overbank sediment deposition. The ¹³⁷Cs approach requires only a single site visit and minimum sample preparation. Furthermore, it is capable of providing information on spatial patterns of sediment deposition on floodplains, which is needed to improve our understanding of the processes involved in overbank flow and sediment deposition. This paper reviews the basis for using ¹³⁷Cs measurements in floodplain sedimentation studies and presents improved procedures for interpreting ¹³⁷Cs profiles in floodplain sediments and for obtaining estimates of sedimentation rates from single measurements of the total. ¹³⁷Cs inventories of bulk sediment cores. The results obtained from a case study undertaken on the floodplain of the River Stour, Dorset, UK, are presented.     

Spatial and vertical distribution of <Superscript>137</Superscript>Cs in soils in the erosive area of southeastern Serbia (Pčinja and South Morava River Basins)

Purpose

The area of southeastern Serbia, the P?inja and South Morava River Basins, is under the influence of very strong erosion, and the aim of this study was to investigate the vertical and spatial distribution of the ¹³⁷Cs in the eroded soils of this area.

Materials and methods

Vertical soil profiles were collected with 5-cm increments from the uppermost layer down to 20, 25, 30, 40, and 50 cm of depth, depending on the thickness of the soil layers, i.e., down to the underlying parent rocks. Measurements of ¹³⁷Cs activity concentration were performed by using the HPGe gamma-ray spectrometer ORTEC-AMETEK (34 % relative efficiency and high resolution 1.65 keV at 1.33 MeV for ⁶⁰Co), from its gamma-ray line at 661.2 keV.

Results and discussion

The mean ¹³⁷Cs activity concentration across all 18 soil profiles (for all soil layers) was found to be 20 Bq kg^?1. In the greatest number of soil profiles, the ¹³⁷Cs activity concentration was generally highest in the first soil layer (0–5 cm) and decreased with soil depth, while in a few soil profiles, the peak of either the ¹³⁷Cs activity concentration occurred in the second soil layer (5–10 cm) or the ¹³⁷Cs activity concentration was almost equal throughout the entire soil profile. The mean ¹³⁷Cs activity concentration in the first soil layer (0–5 cm) was found to be 61 Bq kg^?1, and the high coefficient of variation of 92 % pointed out high spatial variability and large range of the ¹³⁷Cs activity concentrations in the study area.

Conclusions

The obtained results indicate that in the greatest number of soil profiles, ¹³⁷Cs is present in the upper layers, with concentration decreasing with depth, as is typical in uncultivated soil. Its spatial distribution was very uneven among the surface soil layers of the investigated sites. One of the main reasons for such pattern of ¹³⁷Cs in the study area may be soil erosion. Additional investigations which would support this hypothesis are required.

     

Spatial Distribution of 137CS in Forest SOils of Switzerland

In the framework of the second Swiss forest soil inventory, ¹³⁷Cs-activity from 172 sites was measured systematically for the first time in the topmost soil layer (0–5 cm) and represented on a map. The spatial distribution of ¹³⁷Cs contamination was similar to the pattern observed in 1986 from dose equivalent measurements following the Chernobyl nuclear power plant accident. Forest soils from regions with high precipitation in 1986 showed a higher ¹³⁷Cs activity than regions with low precipitation. At sites with high caesium activities it was possible to discriminate between ¹³⁷Cs originating from global fallout of the fifties and sixties and ¹³⁷Cs from the Chernobyl accident. The results indicate that radiocaesium persists in the top soil layers and is recycled in forest ecosystems.     

137Cs tracing of the spatial patterns in soil redistribution,organic carbon and total nitrogen in the southeastern Tibetan Plateau

The southeastern Tibetan Plateau, which profoundly affects East Asia by helping to maintain the stability of climate systems, biological diversity and clean water, is one of the regions most vulnerable to water erosion, wind erosion, tillage erosion, freeze–thaw erosion and overgrazing under global climate changes and intensive human activities. Spatial variations in soil erosion in terraced farmland (TL), sloping farmland (SL) and grassland (GL) were determined by the ¹³⁷Cs tracing method and compared with spatial variations in soil organic carbon (SOC) and total nitrogen (total N). The ¹³⁷Cs concentration in the GL was higher in the 0–0.03 m soil layer than in the other soil layers due to weak migration and diffusion under low precipitation and temperature conditions, while the ¹³⁷Cs concentration in the soil layer of the SL was generally uniform in the 0–0.18 m soil layer due to tillage-induced mixing. Low ¹³⁷Cs inventories appeared at the summit and toe slope positions in the SL due to soil loss by tillage erosion and water erosion, respectively, while the highest ¹³⁷Cs inventories appeared at the middle slope positions due to soil accumulation under relatively flat landform conditions. In the GL, the ¹³⁷Cs data showed that higher soil erosion rates appeared at the summit due to freeze–thaw erosion and steep slope gradients and at the toe slope position due to wind erosion, gully erosion, freeze–thaw erosion and overgrazing. The ¹³⁷Cs inventory generally increased from upper to lower slope positions within each terrace (except the lowest terrace). The ¹³⁷Cs data along the terrace toposequence showed abrupt changes in soil erosion rates between the lower part of the upper terrace and the upper part of the immediate terrace over a short distance and net deposition on the lower and toe terraces. Hence, tillage erosion played an important role in the soil loss at the summit slope positions of each terrace, while water erosion dominantly transported soil from the upper terrace to the lower terrace and resulted in net soil deposition on the flat lower terrace. The SOC inventories showed similar spatial patterns to the ¹³⁷Cs inventories in the SL, TL and GL, and significant correlations were found between the SOC and ¹³⁷Cs inventories in these slope landscapes. The total N inventories showed similar spatial patterns to the inventories of ¹³⁷Cs and SOC, and significant correlations were also found between the total N and ¹³⁷Cs inventories in the SL, TL and GL. Therefore, ¹³⁷Cs can successfully be used for tracing soil, SOC and total N dynamics within slope landscapes in the southeastern Tibetan Plateau.     

Role of plants in the spatial differentiation of <Superscript>137</Superscript>Cs and <Superscript>90</Superscript>Sr statuses on the aggregate level

The increased concentration of an element in plant biomass compared to the soil mass is an essential condition for the differentiated spatial distribution and status of the element on the aggregate level. Two forms of this differentiation have been revealed for ¹³⁷Cs and ⁹⁰Sr. Transfer of ¹³⁷Cs from plant roots and concentration on the surface of soil aggregates have been established experimentally. Indirect data also point to the potential localization of ¹³⁷Cs on the surface of intraaggregate pores. The effect of radionuclide concentrating on the outer and inner surfaces of aggregates is due to the rapid and strong fixation of cesium microamounts by mineral soil components. ¹³⁷Cs from the surface of aggregates is more available for the repeated uptake by plant roots than from the intraped mass. The distortion of this spatial differentiation mainly occurs during the reaggregation of soil mass, which in turn decreases the availability of the radionuclide to plants. For ⁹⁰Sr, its elevated concentration in the form of organic residues has been revealed in the inter- and intraaggregate pore space. However, due to the high diffusion rate, ⁹⁰Sr is relatively rapidly (during several months under pot experimental conditions) redistributed throughout the entire volume of soil aggregates and its major part gradually passes into the phase of humic compounds, to which the radionuclide is bound by exchange sorption. The high level of the next root uptake (higher than for ¹³⁷Cs by one to two orders of magnitude) favors the permanent renewal of loci with increased ⁹⁰Sr concentrations in the inter- and intraaggregate pore space in the form of plant residues.     

Validating the use of Cs measurements to estimate rates of soil redistribution by wind

Wind erosion has degraded over one-half billion hectares of land worldwide. ¹³⁷Cesium (¹³⁷Cs) has been used as a tracer to study long-term rates of soil redistribution by water and, to a lesser extent, by wind. Early studies assumed that the decline in ¹³⁷Cs activity for a potentially eroded soil relative to that for an uneroded soil was linearly proportional to soil loss. More recently, models have emerged that consider the effects of soil cultivation and the particle surface area-dependent partitioning of ¹³⁷Cs on soils. We investigated the partitioning of ¹³⁷Cs in wind-eroded sediments and with soil surface samples sieved into contiguous ranges of particle sizes. We also compared the ¹³⁷Cs activities and stratification of several adjacent soils with known wind erosion and deposition histories. Finally, we tested ¹³⁷Cs-based soil loss models with measured data from sites with documented histories. ¹³⁷Cs activities and mean particle diameters of aeolian samples agreed well with the ¹³⁷Cs activities and respective mean diameters of the sieved surface soil samples. Good agreement between model estimations and measured data indicated that ¹³⁷Cs models developed to estimate soil redistribution by water were also applicable to soil redistribution by wind provided that the models contained an appropriate particle size correction parameter.     

Forms and rates of release of 137Cs in two peat soils

Cation exchange resin saturated with H⁺ and Ca²⁺ was used to extract ¹³⁷Cs from peat soil at two sites in Britain affected by ^l37Cs deposition following the Chernobyl accident. The technique identified three classes of ¹³⁷Cs, similar to those observed for K⁺ in soils: ‘Fast’, ‘Intermediate’ and ‘Slow’. These classes are probably related to the selectivity for ¹³⁷Cs of the cation exchange sites on the organic matter and the clay minerals, and to the structure of the soil. With one exception, most ¹³⁷Cs was in the ‘Slow’ form and was only very slowly released to the resins, if at all. However, there was enough ^l37Cs in the ‘Fast’ and ‘Intermediate’ forms to contaminate pasture and thus grazing animals for some years. Based on the resin technique, it is estimated that contamination will persist for several decades in uplands contaminated at these activity concentrations.     

Relating Intensity of Soil Redistribution to Land Use Changes in Abandoned Pyrenean Fields Using Fallout Caesium‐137

Fallout caesium‐137 has been used to trace soil redistribution in abandoned fields located in the Central Spanish Pyrenees. A total of 28 fields with different lengths, slope angles and time since abandonment were selected on a representative south‐facing slope of the Estarrún valley. The local reference inventory and the magnitude and spatial distribution of ¹³⁷Cs inventories within these fields were documented and used as a basis for assessing patterns of soil redistribution. The local reference inventory was estimated to be 4,500 Bqm⁻². Within the fields, the average ¹³⁷Cs inventory at the top of the slope was 3,920 Bqm⁻², and accumulation of soil at the bottom of the slopes was demonstrated by an average ¹³⁷Cs inventory of 5,320 Bqm⁻². Deviations from the reference inventory were highest for fields with the longest slopes that had been abandoned for less than 30 years. Here, increases in the ¹³⁷Cs inventory, relative to the reference inventory, in excess of 20% were found at the bottom of the slopes. Considering all the fields and all geomorphic positions within the fields, the greatest ¹³⁷Cs losses and gains were found in the fields with the longest duration of abandonment, indicating more intense soil redistribution. Irrespective of the timing of abandonment, the ranges of ¹³⁷Cs inventories in the fields were found to be proportional to the water erosion index. The ¹³⁷Cs technique demonstrated that patterns of sediment redistribution were closely related to the topographic and physiographic characteristics of the slopes. Copyright © 2017 John Wiley & Sons, Ltd.     

Influence of plowing on the depth distribution of various radionuclides in the soil

The present work deals with a comparison of the vertical distribution of ¹³⁷Cs, ¹³⁴Cs, ¹⁰⁶Ru, ¹²⁵Sb, and ⁹⁰Sr at two agricultural sites in Styria (Austria) in the first two years after the Chernobyl fallout. Three months after deposition the Chernobyl derived radionuclides had their maximum concentrations in the first cm. Detectable amounts, however, had penetrated down to a depth of 12 cm (Stagno-Dystric Gleysol, site A) and 20 cm (Dystric Cambisol, site B). Significant differences between the two sites were observed after the first plowing. At site A a new concentration maximum at 15 to 18 cm depth was observed due to an extreme turnover effect. Even the second plowing in 1988 did not yield a homogeneous radionuclide distribution over the tillage depth. At site B the furrow slice was twisted only 60° against the slope gradient. This resulted in a slight mixing in the first 12 cm. From this it may be concluded that plowing does not lead to a thorough mixing in any case. At least two or three plowing steps may be needed to obtain an uniform nuclide distribution at certain sites.     

Detailed early measurements of the fallout in Sweden from the chernobyl accident

Low-volume samplers collecting ambient aerosols in two size fractions have been used to collect radioactivity from the Chernobyl accident. The samplers were situated near light-houses on the east coast of Sweden and samples were collected during consecutive 12-hr periods. Activity concentrations of ⁹⁵Zr, ⁹⁵Nb, ^{103, 106}Ru, ¹³¹I, ^{134, 136, 137}Cs, ¹⁴⁰Ba, ¹⁴⁰La, ^141,144Ce, and ²³⁹Np were measured with a Ge(Li) detector. The transportation time between Chernobyl and the two sampling sites is in good agreement with times calculated from air mass trajectories. The main part of the radioactivity was found on particles with an aerodynamic diameter of less than 2 μm.