Caesium-137 fallout depth distribution in different soil profiles and significance for estimating soil erosion rate

Caesium-137 (¹³⁷Cs) has been widely used for the determination of soil erosion and sediment transport rate. However, depth distribution patterns of ¹³⁷Cs in the soil profile have not been considered. As a result, the erosion rates may be over-estimated or underestimated. This paper presents the depth distribution of ¹³⁷Cs fallout in different soil profiles using published data. Three types of depth distribution functions of ¹³⁷Cs are given by using statistical regression methods, the exponential type, the peak type and the decreasing type (including uniform distribution). Relationships between ¹³⁷Cs loss and soil erosion rate are given by introducing the regression functions. The influence of depth distribution of ¹³⁷Cs on the estimation of the soil erosion rate was simulated. Simulation results showed that very different soil erosion rates could be deduced for different depth distributions when ¹³⁷Cs loss is the same, which indicates that the depth distribution pattern should be considered when soil erosion is estimated by using ¹³⁷Cs. Simulation results also suggested that it is most important to determine the depth distribution of ¹³⁷Cs near the soil surface and the annual relative loss of ¹³⁷Cs by using the depth distribution of ¹³⁷Cs as a criterion to estimate the soil erosion rate.     

利用137Cs示踪技术评价东北黑土侵蚀和沉积过程

Soil and water losses through erosion have been serious in the black soil region of Northeast China. Therefore, a sloping cultivated land in Songnen Plain was selected as a case study to： 1） determine the ^137Cs reference inventory in the study area; 2） calculate erosion and deposition rates of black soil on different slope locations; 3） conduct a sensitivity analysis of some model parameters; and 4） compare overall outputs using four different models. Three transects were set in the field with five slope locations for each transect, including summit, shoulder-slope, back-slope, foot-slope, and toe-slope. Field measurements and model simulation were used to estimate a bomb-derived ^137Cs reference inventory in the study area. Soil erosion and deposition rates were estimated using four ^137Cs models and percentage of ^137Cs loss/gain. The ^137Cs reference value in the study area was 2 232.8 Bq m^-2 with ^137Cs showing a clear topographic pattern, decreasing from the summit to shoulder-slope, then increasing again at the foot-slope and reaching a maximum at the toe-slope, Predicted soil redistribution rates for different slope locations varied. Among models, the Yang Model （YANG-M） overestimated erosion loss but underestimated deposition. However, the standard mass balance model （MBM1） gave predictions similar to a mass balance model incorporating soil movement by tillage （MBM2）. Sensitivity analysis of the proportion factor and distribution pattern of ^137Cs in the surface layer demonstrated the impact of ^137Cs enrichment on calculation of the soil erosion rate. Factors influencing the redistribution of fallout ^137Cs in landscape should be fully considered as calculating soil redistribution rate using ^137Cs technique.     

植被覆盖和雨强对附着在沉积物上的养分流失, 泥沙颗粒组成及体积分形维数的影响

Vegetation and rainfall are two important factors affecting soil erosion and thus resulting in nutrient loss in the Chinese Loess Plateau.A field experiment was conducted to investigate the effects of rainfall intensities(60,100 and 140 mm h-1) and vegetation(Caragana korshinskii) coverages(0%,30% and 80%) on soil loss,nutrient loss,and the composition and volume fractal dimension of eroded sediment particles under simulated rainfall conditions.The results showed that vegetation cover,rainfall intensity and their interaction all had significant effects on sediment transport and the sedimentbound nutrient loss.Higher rainfall intensity and lower coverage led to higher sediment and nutrient losses.Positive linear relationships were observed between soil loss and nutrient loss.The treatments showed more significant effects on the enrichment ratio(ER) of nitrogen(ERN) than organic matter(EROM) and phosphorus(ERP).Compared with the original surface soil,the eroded sediment contained more fine particles.Under the same coverage,the clay content significantly decreased with increasing rainfall intensity.The ER of sediment-bound nutrients was positively correlated with that of clay,suggesting that the clay fraction was preferentially eroded and soil nutrients were mainly adsorbed onto or contained within this fraction.There were increments in the fractal dimension of the sediment particles compared to that of the original surface soil.Moreover,the fractal dimension was positively correlated with clay,silt,and sediment-bound OM,N,and P contents,whereas it was negatively correlated with sand content.This study demonstrated that fractal dimension analysis can be used to characterize differences in particle-size distribution and nutrient loss associated with soil erosion.     

利用137Cs示踪农业耕作土壤侵蚀速率的定量模型

建立了一个根据农业耕作土壤剖面中^137Cs的损失量与土壤侵蚀量之间关系的定量模型,在假设^137Cs在耕层中得到充分的混合而变得均一的基础上,根据质量平衡模型推导而成,模型显示^137Cs的衰变常数,年沉降分量,耕层厚和采样年份对年平均土壤侵蚀速率都有重大影响,模型结果还说明,^137Cs的损失量与年平均土壤侵蚀量之间的关系既非线性关系亦非指数关系,而是一种复杂的曲线关系。     

桑干河流域淤地坝沉积泥沙特征及其来源解析

[目的]为查明桑干河流域的泥沙主要策源地和侵蚀产沙变化。[方法]选取阳原县高墙乡典型淤地坝沉积泥沙为研究对象,利用复合指纹识别技术,测定沉积泥沙及其源地的土壤粒径、SOC、TN、¹³⁷Cs、低频质量磁化率等9种指纹因子,研究了不同淤积阶段的泥沙策源地及坝控小流域侵蚀产沙演变规律。[结果](1)沉积泥沙中¹³⁷Cs平均含量较低,与沟壁土壤无显著差异(p>0.05),但极显著小于林草地和耕地的¹³⁷Cs含量(p<0.01),这指示淤地坝沉积泥沙主要来源于沟壁;(2)由于沟壁中大部分¹³⁷Cs含量低于检出限,¹³⁷Cs较好地指示泥沙主要来源沟谷地中的沟壁,但难以用于小流域多种策源地的判别,经Kruskal-Wallis H非参数检验和多元逐步判别分析筛选,确定TN+X_lfb+SOC构成最佳指纹因子组合,有效地判别小流域2006—2017年泥沙源地的平均贡献率为沟壁(82.68%±8.20%)>耕地(15.36%±8.46%)>林草地(1....     

137Cs tracing of the spatial patterns in soil redistribution,organic carbon and total nitrogen in the southeastern Tibetan Plateau

The southeastern Tibetan Plateau, which profoundly affects East Asia by helping to maintain the stability of climate systems, biological diversity and clean water, is one of the regions most vulnerable to water erosion, wind erosion, tillage erosion, freeze–thaw erosion and overgrazing under global climate changes and intensive human activities. Spatial variations in soil erosion in terraced farmland (TL), sloping farmland (SL) and grassland (GL) were determined by the ¹³⁷Cs tracing method and compared with spatial variations in soil organic carbon (SOC) and total nitrogen (total N). The ¹³⁷Cs concentration in the GL was higher in the 0–0.03 m soil layer than in the other soil layers due to weak migration and diffusion under low precipitation and temperature conditions, while the ¹³⁷Cs concentration in the soil layer of the SL was generally uniform in the 0–0.18 m soil layer due to tillage-induced mixing. Low ¹³⁷Cs inventories appeared at the summit and toe slope positions in the SL due to soil loss by tillage erosion and water erosion, respectively, while the highest ¹³⁷Cs inventories appeared at the middle slope positions due to soil accumulation under relatively flat landform conditions. In the GL, the ¹³⁷Cs data showed that higher soil erosion rates appeared at the summit due to freeze–thaw erosion and steep slope gradients and at the toe slope position due to wind erosion, gully erosion, freeze–thaw erosion and overgrazing. The ¹³⁷Cs inventory generally increased from upper to lower slope positions within each terrace (except the lowest terrace). The ¹³⁷Cs data along the terrace toposequence showed abrupt changes in soil erosion rates between the lower part of the upper terrace and the upper part of the immediate terrace over a short distance and net deposition on the lower and toe terraces. Hence, tillage erosion played an important role in the soil loss at the summit slope positions of each terrace, while water erosion dominantly transported soil from the upper terrace to the lower terrace and resulted in net soil deposition on the flat lower terrace. The SOC inventories showed similar spatial patterns to the ¹³⁷Cs inventories in the SL, TL and GL, and significant correlations were found between the SOC and ¹³⁷Cs inventories in these slope landscapes. The total N inventories showed similar spatial patterns to the inventories of ¹³⁷Cs and SOC, and significant correlations were also found between the total N and ¹³⁷Cs inventories in the SL, TL and GL. Therefore, ¹³⁷Cs can successfully be used for tracing soil, SOC and total N dynamics within slope landscapes in the southeastern Tibetan Plateau.     

Investigating the effects of afforestation on soil erosion and sediment mobilisation in two small catchments in Southern Italy

Annual soil losses in southern Italy can exceed 100–150 t ha^− 1 year^− 1. Where erosion on agricultural land is particularly severe, land use change and afforestation are frequently seen as the most appropriate means of reducing erosion risk. However, the overall effectiveness of afforestation in reducing soil erosion remains uncertain, due to the poor development of the forest cover in some areas, leading to significant areas with sparse tree cover, and the erosional impact of forest harvesting, which commonly involves clearcutting. The study reported here addresses this uncertainty and focuses on two small catchments (W2 and W3) located in Calabria, southern Italy, for which measurements of suspended sediment yield are available. Both the catchments originally supported a rangeland vegetation cover and they were planted with eucalyptus trees in 1968. Currently, only catchment W3 supports a continuous forest cover. In catchment W2 the forest cover is discontinuous and there is a significant area of the catchment (ca. 20%) where the tree cover is sparse and the vegetation cover is dominated by natural grasses. Two additional erosion plots were established within catchment W2 in 1991, in order to explore the effect of the density of the tree cover on soil erosion. Information on the sediment yields from the two catchments and the plots for 10 storm events that occurred during the period December 2005–December 2006 and associated information on the ¹³⁷Cs and excess ²¹⁰Pb of the sediment, have been used to investigate the effectiveness of afforestation in reducing sediment mobilisation and net soil loss from the catchments involved. The results demonstrate that the areas of greatest soil loss are associated with the slopes where the tree cover is discontinuous, and that forest harvesting by clearcutting causes significant short-term increases in sediment mobilisation and sediment yield. These findings, which are consistent with previous work undertaken within the same area, emphasize the importance of vegetation cover density in influencing rates of soil loss in the study catchments. The study also provided a useful demonstration of the potential for using measurements of the ¹³⁷Cs and ²¹⁰Pb_ex content of sediment, in combination with more traditional sediment monitoring, to investigate sediment sources and to compare the sediment dynamics of catchments subjected to different land management practices.     

A tracer budget quantifying soil redistribution on hillslopes after forest harvesting

Managing the impacts of erosion after forest harvesting requires knowledge of erosion sources; rates of sediment transport and storage; as well as losses from the system. We construct a tracer-based (¹³⁷Cs) sediment budget to quantify these parameters. The budget shows significant redistribution, storage and transport of sediment between landscape elements and identifies the snig tracks and log landings as the major impact sites in the catchment. Annual sediment losses from them were estimated to be 25±11 and 101±15 t ha⁻¹ year⁻¹, respectively, however, it is probable that most of this is due to mechanical displacement of soil at the time of harvesting. The budget showed greatest net transport of material occurring from snig tracks; representing some 11±4% of the ¹³⁷Cs budget. Of the latter amount, 18%, 28% and 43% was accounted for within the cross banks, filter strip and General Harvest Area (GHA), respectively. The ¹³⁷Cs budget also showed the GHA to be a significant sediment trap. The filter strip played a fundamental role in the trapping of material generated from the snig tracks, the mass delivery to them from this source was calculated to be 1.7±0.6 kg m² year⁻¹. Careful management of these remains critical. Overall we could account for 97±10% of ¹³⁷Cs. This retention suggests that (within errors) the overall runoff management system of dispersing flow (and sediment) from the highly compacted snig tracks, by cross banks, into the less compacted (and larger area) GHA and filter strips has effectively retained surface soil and sediment mobilised as a result of harvesting at this site.     

三峡库区紫色土坡耕地土壤侵蚀的137Cs示踪研究

坡耕地是三峡库区的重点水土流失区和河流泥沙的主要来源地.采用~(137)Cs示踪技术对三峡库区紫色土坡耕地的土壤侵蚀速率进行了定量研究.结果表明,新政小流域的~(137)Cs本底值为1 420.9 Bq/m~2;平均坡度为11.4°的缓坡耕地的~(137)Cs面积活度介于398.5～1 649.6 Bq/m~2之间,坡长加权平均值为816.0Bq/m~2;采用改进的简化质量平衡模型计算了坡耕地的土壤侵蚀速率,结果得出该坡地的土壤侵蚀模数介于-3 358.8～4 937.4 t/(km~2·a),其加权平均值为1 294.6 t/(km~2·a).受犁耕作用的影响,坡耕地两个坡段的土壤侵蚀速率随坡长增加大致都呈下降趋势,并在坡段下方出现了堆积.坡耕地土壤侵蚀速率不高的原因,一方面是由于所研究坡耕地属于缓坡,坡度较小,另一方面则是由于当地农民总结出了一套有效防止水土流失的耕作方式,使得土壤侵蚀强度大大降低.     

Validating the use of Cs measurements to estimate rates of soil redistribution by wind

Wind erosion has degraded over one-half billion hectares of land worldwide. ¹³⁷Cesium (¹³⁷Cs) has been used as a tracer to study long-term rates of soil redistribution by water and, to a lesser extent, by wind. Early studies assumed that the decline in ¹³⁷Cs activity for a potentially eroded soil relative to that for an uneroded soil was linearly proportional to soil loss. More recently, models have emerged that consider the effects of soil cultivation and the particle surface area-dependent partitioning of ¹³⁷Cs on soils. We investigated the partitioning of ¹³⁷Cs in wind-eroded sediments and with soil surface samples sieved into contiguous ranges of particle sizes. We also compared the ¹³⁷Cs activities and stratification of several adjacent soils with known wind erosion and deposition histories. Finally, we tested ¹³⁷Cs-based soil loss models with measured data from sites with documented histories. ¹³⁷Cs activities and mean particle diameters of aeolian samples agreed well with the ¹³⁷Cs activities and respective mean diameters of the sieved surface soil samples. Good agreement between model estimations and measured data indicated that ¹³⁷Cs models developed to estimate soil redistribution by water were also applicable to soil redistribution by wind provided that the models contained an appropriate particle size correction parameter.     

Validating the Use of 137Cs Measurements to Derive the Slope Component of the Sediment Budget of a Small Rangeland Catchment in Southern Italy

The sediment budget is a key concept and tool for characterizing the mobilization, transfer and storage of fine sediment within a catchment. Caesium‐137 measurements can provide valuable information on gross and net erosion rates associated with sheet and rill erosion that can be used to establish the slope component of a catchment sediment budget. However, there is a need to validate the use of ¹³⁷Cs measurements for this purpose, because their reliability has sometimes been questioned. The study reported focuses on a small (3·04 ha) steepland (mean slope 37%) catchment in Southern Italy. It exploits the availability of information on the medium‐term sediment output from the catchment provided by the construction of a reservoir at its outlet in 1978 and the existence of estimates of soil redistribution rates derived from ¹³⁷Cs measurements made on 68 replicate soil cores collected from the slopes of a substantial proportion of the catchment in 2001, to validate the use of ¹³⁷Cs measurements to construct the slope component of the catchment sediment budget. An additional 50 replicate soil cores were collected from the catchment slopes for ¹³⁷Cs analysis, to complement the data already available. Nine cores collected from the area occupied by the reservoir were used to estimate the mean annual sediment input to the reservoir. In the absence of evidence that the poorly developed channel system in the catchment was either a significant sediment source or sink, it was possible to directly compare the estimate of net soil loss from the catchment slopes (7·33 Mg ha⁻¹ y⁻¹) with the estimate of sediment output from the catchment provided by the reservoir deposits (7·52 Mg ha⁻¹ y⁻¹). Taking account of the uncertainties involved, the close agreement of the two values is seen as providing a convincing validation of the use of ¹³⁷Cs measurements to both estimate soil redistribution rates and as a basis for constructing the slope component of the sediment budget of a small catchment. Copyright © 2015 John Wiley & Sons, Ltd.     

Application of Chernobyl-derived Cs for the assessment of soil redistribution within a cultivated field

Vast areas of Europe were contaminated by the Chernobyl-derived ¹³⁷Cs in April–May 1986. This paper reports a detailed study of the post-fallout ¹³⁷Cs redistribution within a 1 ha field located in the Chasovenkov Verh catchment in the northern part of the Middle-Russian upland. Particular attention was paid to the study of reference inventories. It is shown that the random spatial variability of ¹³⁷Cs is similar within undisturbed and cultivated parts of a flat interfluve. Systematic spatial variability is not essential for a relatively short (200 m) topographical unit with simple relief. The analysis of a soil redistribution pattern within the study field using the Chernobyl ¹³⁷Cs technique demonstrates that it is possible to identify areas of soil loss/gain. This pattern does not reflect soil redistribution for the whole field, because these have been only 12 years since the Chernobyl accident. Net erosion rates based on ¹³⁷Cs method were comparable to soil losses directly measured at the study field.     

Validating erosion rate estimates provided by caesium‐137 measurements for two small forested catchments in Calabria,southern Italy

Increasing concern for problems of soil degradation and the off‐site impacts of accelerated erosion has generated a need for improved methods of estimating rates and patterns of soil erosion by water. The use of environmental radionuclides, particularly ¹³⁷Cs, to estimate erosion rates has attracted increased attention and the approach has been shown to possess several important advantages. However, the use of ¹³⁷Cs measurements to estimate erosion rates introduces one important uncertainty, namely, the need to employ a conversion model or relationship to convert the measured reduction in the ¹³⁷Cs inventory to an estimate of the erosion rate. There have been few attempts to validate these theoretical conversion models and the resulting erosion rate estimates. However, there is an important need for such validation, if the ¹³⁷Cs approach is to be more widely applied and reliance is to be placed on the results obtained. This paper reports the results of a study aimed at validating the use of two theoretical conversion models, namely the exponential depth distribution model and the diffusion and migration model, that have been used in several recent studies to convert measurements of ¹³⁷Cs inventories on uncultivated soils to estimates of soil erosion rates. The study is based on data assembled for two small catchments (1.38 and 1.65 ha) in Calabria, southern Italy, for which measurements of sediment output are available for the catchment outlet. The two catchments differ in terms of the steepness of their terrain, and this difference is reflected by their sediment yields. Because there is no evidence of significant deposition within the two catchments, sediment delivery ratios close to 1.0 can be assumed. It is therefore possible to make a direct comparison between the estimates of the mean annual erosion rates within the two catchments derived from ¹³⁷Cs measurements and the measured sediment outputs. The results of the comparison show that the erosion rate estimates provided by both models are reasonably consistent with the measured sediment yields at the catchment outlets. However, more detailed assessment of the results shows that the validity of the erosion rate estimates is influenced by the magnitude of the erosion rates within the catchment. The exponential depth distribution model appears to perform better for the catchment with higher erosion rates and to overestimate erosion rates in the other catchment. Similarly, the basic migration and diffusion model performs better for the catchment with lower erosion rates and overestimates erosion rates in the other catchment. However, the improved migration and diffusion model appears to perform satisfactorily for both catchments. There is a need for further studies to extend such independent validation of the ¹³⁷Cs technique to other environments, including cultivated soils, and to other conversion models and procedures. Copyright © 2003 John Wiley & Sons, Ltd.     

Dual roles of tillage erosion in lateral SOC movement in the landscape

The facts that the global carbon budget cannot be currently balanced and current estimates of agricultural sources and sinks may be inaccurate, may be linked to unaccounted‐for erosion‐induced changes in soil organic carbon (SOC). A closed landscape with field banks and an open landscape without field banks were selected from two sites located in Jianyang County, Sichuan Province, and Zhongxian County, Chongqing Municipality, respectively. In these landscapes, the role of tillage and water erosion was examined using measurements of soil redistribution in relation to ¹³⁷Cs radionuclide depth‐stratigraphy, to elucidate the mechanism of SOC depth distribution in the soil profile and resultant stocks in agricultural landscapes of terraced field systems. Changes in the ¹³⁷Cs inventory at different landscape positions depend on both ¹³⁷Cs concentrations of individual subsample layers (5‐cm depth) and the vertical extent of ¹³⁷Cs depth distribution in the terrace system with field banks, while the changes are only associated with the vertical extent of ¹³⁷Cs depth distribution in the terrace system without field banks because of similar ¹³⁷Cs concentrations of individual subsample layers. The profile shape of SOC depth distribution exhibits notable differences between the upper and lower parts of the terrace in systems with field banks, but no apparent differences were found in the systems without field banks and the SOC profile shape is similar to that of the upper part of the terrace in systems with field banks. It is suggested that SOC depth distribution in these two types of terraced field systems is controlled by different soil erosion patterns. Tillage erosion playing a dominant role in the process of soil erosion within a landscape can increase SOC stocks. However, SOC depletion takes place in situations where the two processes of tillage and water erosion are both important and tillage erosion acts as a delivery mechanism for water erosion. We conclude that tillage erosion plays a dual role: enhancing carbon storage at depositional positions, and accelerating carbon depletion when combined with water erosion within the same landscape.     

Radio-caesium fixation dynamics: measurement in six Cumbrian soils

Five peat soils and a mineral soil were artificially contaminated with ¹³⁷Cs. Soil solution activity and radio–lability of ¹³⁷Cs were monitored over 709 days to quantify progressive ¹³⁷Cs fixation. The peat soils fixed large amounts of ¹³⁷Cs, but less than the mineral soil did. Distribution coefficients (K_d, cm³ g^?1) ranged from 30 to 5000 at the end of equilibration. A labile ¹³⁷Cs distribution coefficient, K_dt, was estimated by a method involving solid ? solution equilibration in dilute solution. In a separate study several concentrations of KCl were added to soils in increasing concentration both before and after the addition of ¹³⁷Cs. Differences in apparent adsorption strength of radiocaesium indicated that K⁺ induced the collapse of expanded mineral interlayers, thereby trapping ions. It seemed that ^I37Cs adsorbs at sites in the small micaceous clay fraction of the peat soils. The different rates of ¹³⁷Cs adsorption and fixation in the peat and mineral soils, in which the rate of access of ¹³⁷Cs to fixation sites in peat soils is less, seems to have been caused partly by lack of K, and partly by the scarcity of fixation sites.     

Residue cover and rainfall intensity effects on runoff soil organic carbon losses

Soil cover and rainfall intensity (RI) are recognized to have severe impacts on soil erosion and an interaction exists between them. This study investigates the effect of rainfall intensity (RI) and soil surface cover on losses of sediment and the selective enrichment of soil organic carbon (SOC) in the sediment by surface runoff. A field rainfall simulator was used in the laboratory to produce 90 min rainfall events of three rainfall intensities (65, 85 and 105 mm h^− 1) and four cover percentages (0%, 25%, 50% and 75%) on soil material at 9% slope. A strong negative exponential relation was observed between cover percentage and RI on sediment loss under 85 and 105 mm h^− 1 of rain, while under RI of 65 mm h^− 1, the highest sediment loss was observed under 25% cover. Overall, higher RI and lower cover produced higher sediment and consequently higher nutrient loss, but resulted in a lower SOC enrichment ratio (ER_SOC) in the sediment. The amount of runoff sediment rather than the ER_SOC in the sediment was the determinant factor for the amount of nutrients lost. The values of ER_SOC were high and positively correlated with the ER values of particles smaller than 20 µm (p < 0.01). Although the sediment contained substantially more fine fractions (fine silt and clay, < 20 µm), the original soil and runoff sediment were still of the same texture class, i.e. silt clay loam.     

Use of 137Cs measurements to investigate soil erosion on arable fields in the UK: potential applications and limitations

Recent awareness of the potential hazard of soil erosion on arable land in the UK has highlighted the lack of reliable data concerning actual rates of soil loss. This lack of information reflects both a low level of interest, and the lack of a simple and generally applicable method of documenting long-term rates of soil loss. Existing methods involving the use of hazard classification procedures and direct measurement techniques, including erosion plots and field surveys, all possess significant limitations. The use of ¹³⁷Cs measurements to provide information on rates of soil loss and deposition averaged over the past 30 years would appear to offer considerable potential. The results of applying this approach to three arable fields on contrasting soil types in Britain are reported. These results confirm the viability of the technique and its potential for providing information on patterns and rates of erosion and deposition within individual fields and their overall sediment budgets. Limitations include the restricted size of the areas that can be investigated and the need to take account of additional inputs of ¹³⁷Cs derived from the Chernobyl accident.     

Migration and Chemical Availability of 137Cs and 90Sr in SwedishLong-Term Experimental Pastures

Migration and chemical availability of ¹³⁷Cs and⁹⁰Sr in the long-term was studied on a36-yr-old deposition experiment on pastureconsisting of a sandy soil and a clay soil,contaminated in 1961 with radionuclides in aqueoussolution. Comparisons were made with a study of thesame soils in 1967. Soil samples to 55 cm depth wereanalysed for ¹³⁷Cs and ⁹⁰Sr to establish thevertical distribution. Chemical availability wasstudied using sequential extractions with H₂O,NH₄Ac, NH₂OH·HCl, H₂O₂ andHNO₃. Both ¹³⁷Cs and ⁹⁰Sr were found atall depths in both soil types. Cs-137 waspredominantly retained within the upper 10 cm (70%)in both soils. For ⁹⁰Sr, the soils differedsignificantly, retention within the upper 10 cm was27% in sandy soil and 47% in clay soil. Migrationsince 1967 was faster in the sandy soil for bothnuclides. More than 95% of ¹³⁷Cs was bound inthe acid-digestible and residual fractions in bothsoils. The residual fraction was larger in clay soil.⁹⁰Sr was highly available in both soils. Noresidual fraction was found, and the easilyexchangeable fraction was 63–75%.     

A preliminary assessment of the potential for using Pbex measurement to estimate soil redistribution rates on cultivated slopes in the Sichuan Hilly Basin of China

In order to assess its potential for estimating soil redistribution rates, the naturally occurring fallout radionuclide ²¹⁰Pb_ex has been used in parallel with ¹³⁷Cs, derived from the atmospheric testing of nuclear weapon testing in the 1950s to 1970s, to estimate rates of soil redistribution on a sloping field with traditional erosion control measures located near Jiajia Village, Jianyang County, in the Sichuan Hilly Basin of China. The local ²¹⁰Pb_ex reference inventory of 12,860 Bq m^− 2 is higher than those reported for many other areas of the world and may reflect the influence of cloudy weather in preventing ²¹⁰Pb released to the atmosphere across the local region moving up into the upper troposphere, where is would be more widely dispersed. The mean ²¹⁰Pb_ex and ¹³⁷Cs inventories measured in cores collected from the upper part of the field with an average slope of 10° were 8028 Bq m^− 2 and 993 Bq m^− 2, respectively, and the equivalent values for the lower part of the field, where the slopes are steeper (20°) were 11,388 Bq m^− 2 and 1299 Bq m^− 2. The pattern of post-fallout ²¹⁰Pb_ex and ¹³⁷Cs redistribution on the sloping field reflects not only the effects of water erosion and redistribution by tillage, but also the local traditional practice of “Tiaoshamiantu”, whereby sediment trapped in the ditches is returned to the fields by the farmer. The estimates of annual rates of soil loss provided by the ²¹⁰Pb_ex measurement are closely comparable with those derived from the ¹³⁷Cs measurements and are consistent with existing knowledge for the study area. The results obtained from this study confirm the potential for using ²¹⁰Pb_ex measurement to estimate soil erosion rates over medium-term timescale of 50–100 years. By combining the estimates of erosion rates provided by the ²¹⁰Pb_ex and ¹³⁷Cs measurements, the weighted mean net soil loss was estimated to be 48.7 t ha^− 1 year^− 1 from the upper subfield and 16.9 t ha^− 1 year^− 1 from the lower subfield. These rates are considerably lower than the erosion rates obtained from runoff plot measurements in the local area. It is suggested that the traditional erosion control practices and the practice of “Tiaoshamiantu” have a significant effect in reducing soil loss and conserving valuable cultivated soil on sloping fields in the Sichuan Hilly Basin.     

应用137Cs示踪技术估算土壤侵蚀的若干问题探讨

[目的]探讨用~(137)Cs示踪技术估算土壤侵蚀量方法(以下简称"~(137)Cs示踪方法")所存在的几个关键问题,促进该方法的标准化和系统化。[方法]对大量已发表的相关文献进行分析,根据作者的研究经验,归纳出~(137)Cs示踪方法在实践应用中所存在的核心问题。[结果]~(137)Cs示踪方法中关于~(137)Cs在空间是均匀分布的假设存在不合理性,不能直接用于定量估算单钻点取样的土壤侵蚀量。~(137)Cs活度的空间变化存在随机性的成分。敏感度和不确定性分析结果证明~(137)Cs活度的空间随机变化量是~(137)Cs示踪方法不确性的最大来源。[结论]可以用多钻点样本平均值来减少~(137)Cs随机变化量所引起的侵蚀估算误差。以统计学为基础的试验设计和采取独立样本的办法可以消除该误差。虽然~(137)Cs模型已被广泛应用,但由于缺乏长期观测资料诸多模型还处在理论研究阶段,没有得到严格的验证和评判。因为不同模型估算的侵蚀量差别甚大,模型验证和筛选对该方法的成功运用至关重要。