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台州市典型电子垃圾拆解场地周边农田土壤重金属污染特征和来源解析
引用本文:郑宇娜,刘鹏,刘金河,周长瑞,王琪,冯美云,刘冠宏,朱旭东,林匡飞.台州市典型电子垃圾拆解场地周边农田土壤重金属污染特征和来源解析[J].农业环境科学学报,2022,41(7):1442-1451.
作者姓名:郑宇娜  刘鹏  刘金河  周长瑞  王琪  冯美云  刘冠宏  朱旭东  林匡飞
作者单位:华东理工大学资源与环境工程学院, 化学工程环境风险评估与控制国家环境保护重点实验室, 上海 200237
基金项目:国家科技重大专项(2019YFC1803701)
摘    要:为分析台州市电子垃圾拆解场地周边农田土壤中重金属污染特征和来源贡献,在2021年3月采集研究区230个表层(0~20cm)农田土壤,测定了样品中9种重金属(Cr、Co、Ni、Cu、Zn、As、Cd、Hg和Pb)元素含量。通过污染负荷指数(PLI)和潜在生态风险指数(RI)分析重金属的生态风险,并利用地统计、多变量统计和...

关 键 词:农田土壤  电子垃圾  重金属  空间分布  源解析  风险评价
收稿时间:2021/12/1 0:00:00

Pollution characteristics and source analysis of heavy metals in farmland soils around the e-waste dismantling sites in Taizhou City, China
ZHENG Yun,LIU Peng,LIU Jinhe,ZHOU Changrui,WANG Qi,FENG Meiyun,LIU Guanhong,ZHU Xudong,LIN Kuangfei.Pollution characteristics and source analysis of heavy metals in farmland soils around the e-waste dismantling sites in Taizhou City, China[J].Journal of Agro-Environment Science( J. Agro-Environ. Sci.),2022,41(7):1442-1451.
Authors:ZHENG Yun  LIU Peng  LIU Jinhe  ZHOU Changrui  WANG Qi  FENG Meiyun  LIU Guanhong  ZHU Xudong  LIN Kuangfei
Institution:State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resources and Environmental Engineering, East China University of Science and Technology, Shanghai 200237, China
Abstract:In order to analyze the pollution characteristics and source contributions of heavy metals in farmland soils around the e-waste dismantling sites in Taizhou City, 230 surface (0~20 cm) farmland soils in the study area were collected in March 2021. The contents of heavy metals (Cr, Co, Ni, Cu, Zn, As, Cd, Hg, and Pb) in these soils were determined. The ecological risks of the heavy metals were analyzed using the pollution load index (PLI) and potential ecological risk index (RI). Moreover, the sources of the soil heavy metals in this area were analyzed using the combination of geostatistics, multivariate statistics and PMF modelling. The results showed that the Cd pollution levels of farmland soils around the study area were the highest, the median exceeded the risk screening values for soil contamination of agricultural land, and the exceeding standard rate reached 75.65%. In addition, the exceeding standard rates of Cr and Cu were relatively high, 27.39% and 42.61% respectively. The comprehensive pollution load index indicated that 16.96% and 7.39% of the samples constituted moderate or serious pollution, respectively. Nevertheless, the potential risk indices (55.22% and 34.78%) of the samples were considered moderate and above severe risk, respectively. The comprehensive results of geostatistics, multivariate statistics and PMF modelling showed that the sources of nine heavy metals in these soil samples could be divided into four categories:Co, Cr, and Ni mainly come from natural sources; As mainly comes from agricultural sources; Zn, Cu, Cd, and Pb mainly come from metal smelting sources, concentrating in the farmland soils around historical e-waste dismantling sites; and Hg mainly comes from coal and industrial sources.
Keywords:farmland soil  e-waste  heavy metal  spatial distribution  source apportionment  risk assessment
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