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Atmospheric sulfur deposition for a red soil broadleaf forest in southern China
作者姓名:XU Cheng-Kai  HU Zheng-Yi  CAI Zu-Cong  WANG Ti-Jian  HE Yuan-Qiu  CAO Zhi-Hong
作者单位:[1]StateKeyLaboratoryofSoilandSustainableAgriculture,InstituteofSoilScience,ChineseAcademyofSciences,Nanjing210008(China) [2]DepartmentofAtmosphericScience,NanjingUniversity,Nanjing210093(China)
基金项目:*1Project supported by the National Key Basic Research Support Foundation (NKBRSF) of China (No.1999011805), the Knowledge Innovation Program of Chinese Academy of Sciences (No.ISSASIP0205), the State Key Laboratory of Soil and Sustainable Agriculture, China; and the Scientific Research Foundation for Returned Overseas Chinese Scholars, the State Education Ministry of China.
摘    要:A two-year study in a typical red soil region of Southern China was conducted to determine 1) the dry deposition velocity (Vd) for SO2 and particulate SO4^2- above a broadleaf forest, and 2) atmospheric sulfur fluxes so as to estimate the contribution of various fractions in the total. Using a resistance model based on continuous hourly meteorological data, atmospheric dry sulfur deposition in a forest was estimated according to Va and concentrations of both atmospheric SO2 and particulate SO2^4-. Meanwhile, wet S deposition was estimated based on rainfall and sulfate concentrations in the rainwater. Results showed that about 99% of the dry sulfur deposition flux in the forest resulted from SO2 dry deposition.In addition, the observed dry S deposition was greater in 2002 than in 2000 because of a higher average concentration of SO2 in 2002 than in 2000 and not because of the average dry deposition velocity which was lower for SO2 in 2002. Also,dry SO2 deposition was the dominant fraction of deposited atmospheric sulfur in forests, contributing over 69% of the total annual sulfur deposition. Thus, dry SO2 deposition should be considered when estimating sulfur balance in forest ecological systems.

关 键 词:大气沉降  干燥沉降速度  红土  二氧化硫  

Atmospheric sulfur deposition for a red soil broadleaf forest in southern China
XU Cheng-Kai,HU Zheng-Yi,CAI Zu-Cong,WANG Ti-Jian,HE Yuan-Qiu,CAO Zhi-Hong.Atmospheric sulfur deposition for a red soil broadleaf forest in southern China[J].Pedosphere,2004,14(3):323-330.
Authors:XU Cheng-Kai  HU Zheng-Yi  CAI Zu-Cong  WANG Ti-Jian  HE Yuan-Qiu and CAO Zhi-Hong
Institution:State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008 (China). E-mail: chkxu@issas.ac.cu;State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008 (China). E-mail: chkxu@issas.ac.cu;State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008 (China). E-mail: chkxu@issas.ac.cu;Department of Atmospheric Science, Nanjing University, Nanjing 210093 (China);State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008 (China). E-mail: chkxu@issas.ac.cu;State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008 (China). E-mail: chkxu@issas.ac.cu
Abstract:A two-year study in a typical red soil region of Southern China was conducted to determine 1) the dry deposition velocity (Vd) for SO2 and particulate SO4^2- above a broadleaf forest, and 2) atmospheric sulfur fluxes so as to estimate the contribution of various fractions in the total. Using a resistance model based on continuous hourly meteorological data, atmospheric dry sulfur deposition in a forest was estimated according to Va and concentrations of both atmospheric SO2 and particulate SO2^4-. Meanwhile, wet S deposition was estimated based on rainfall and sulfate concentrations in the rainwater. Results showed that about 99% of the dry sulfur deposition flux in the forest resulted from SO2 dry deposition.In addition, the observed dry S deposition was greater in 2002 than in 2000 because of a higher average concentration of SO2 in 2002 than in 2000 and not because of the average dry deposition velocity which was lower for SO2 in 2002. Also,dry SO2 deposition was the dominant fraction of deposited atmospheric sulfur in forests, contributing over 69% of the total annual sulfur deposition. Thus, dry SO2 deposition should be considered when estimating sulfur balance in forest ecological systems.
Keywords:atmospheric sulfur deposition  dry deposition velocity  particulate SO42-  red soil  SO2
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